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Main Authors: Fan, Haoran, Chen, Yue, Gu, Yuchen, Li, Yuan, Lin, Xi
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2406.17421
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author Fan, Haoran
Chen, Yue
Gu, Yuchen
Li, Yuan
Lin, Xi
author_facet Fan, Haoran
Chen, Yue
Gu, Yuchen
Li, Yuan
Lin, Xi
contents Honeycomb cobalt oxides containing 3$\it{d}$ Co$^{2+}$ ions might realize frustrated magnetism and novel quantum phases. Among candidate materials, Na$_{3}$Co$_{2}$SbO$_{6}$ stands out for its distorted honeycomb lattice and significant in-plane anisotropy, motivating vector-field tuning inside the honeycomb plane. Here we use thermal transport down to the mK regime to study twin-free crystals of Na$_{3}$Co$_{2}$SbO$_{6}$ subject to in-plane vector fields. We find that the thermal conductivity $κ$ never exceeds the heat-transport capability of phonons, rendering its suppression primarily due to phonon scattering off magnetic excitations and/or domain boundaries. The system's field-driven quantum criticality manifests itself as an abundance of magnetic fluctuations hindering the heat transport, which further depends on the field direction in an intriguing manner.
format Preprint
id arxiv_https___arxiv_org_abs_2406_17421
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Phonon Heat Transport and Anisotropic Tuning of Quantum Fluctuations in a Frustrated Honeycomb Magnet
Fan, Haoran
Chen, Yue
Gu, Yuchen
Li, Yuan
Lin, Xi
Strongly Correlated Electrons
Honeycomb cobalt oxides containing 3$\it{d}$ Co$^{2+}$ ions might realize frustrated magnetism and novel quantum phases. Among candidate materials, Na$_{3}$Co$_{2}$SbO$_{6}$ stands out for its distorted honeycomb lattice and significant in-plane anisotropy, motivating vector-field tuning inside the honeycomb plane. Here we use thermal transport down to the mK regime to study twin-free crystals of Na$_{3}$Co$_{2}$SbO$_{6}$ subject to in-plane vector fields. We find that the thermal conductivity $κ$ never exceeds the heat-transport capability of phonons, rendering its suppression primarily due to phonon scattering off magnetic excitations and/or domain boundaries. The system's field-driven quantum criticality manifests itself as an abundance of magnetic fluctuations hindering the heat transport, which further depends on the field direction in an intriguing manner.
title Phonon Heat Transport and Anisotropic Tuning of Quantum Fluctuations in a Frustrated Honeycomb Magnet
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2406.17421