The Origin of Sound Damping in Amorphous Solids: Defects and Beyond

Fuente: arXiv
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Main Authors: Flenner, Elijah, Szamel, Grzegorz
Format: Preprint
Published: 2024
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author Flenner, Elijah
Szamel, Grzegorz
author_facet Flenner, Elijah
Szamel, Grzegorz
contents Comprehending sound damping is integral to understanding the anomalous low temperature properties of glasses. After decades of theoretical and experimental studies, Rayleigh scattering scaling of the sound attenuation coefficient with frequency, $Γ\sim ω^{d+1}$, became generally accepted when quantum and finite temperature effects can be neglected. Rayleigh scaling invokes a picture of scattering from defects. However, it is unclear how to define glass defects, or even if defects are necessary for Rayleigh scaling. Here we determine a particle level contribution to sound damping in the Rayleigh scaling regime. We find that there are areas in the glass that contribute more to sound damping than other areas over a range of frequencies, which allows us to define defects. We show that over a range of glass stability, sound damping scales linearly with the fraction of particles in the defects. However, sound is still attenuated in ultra-stable glasses where no defects are identified. We show that sound damping in these glasses is due to nearly uniformly distributed non-affine, microscopic forces that arise after macroscopic deformations of non-centrosymetric structures. To fully understand sound attenuation in glasses one has to consider contributions from defects and a defect-free background, which represents a new paradigm of sound damping in glasses.
format Preprint
id arxiv_https___arxiv_org_abs_2406_18667
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle The Origin of Sound Damping in Amorphous Solids: Defects and Beyond
Flenner, Elijah
Szamel, Grzegorz
Disordered Systems and Neural Networks
Materials Science
Comprehending sound damping is integral to understanding the anomalous low temperature properties of glasses. After decades of theoretical and experimental studies, Rayleigh scattering scaling of the sound attenuation coefficient with frequency, $Γ\sim ω^{d+1}$, became generally accepted when quantum and finite temperature effects can be neglected. Rayleigh scaling invokes a picture of scattering from defects. However, it is unclear how to define glass defects, or even if defects are necessary for Rayleigh scaling. Here we determine a particle level contribution to sound damping in the Rayleigh scaling regime. We find that there are areas in the glass that contribute more to sound damping than other areas over a range of frequencies, which allows us to define defects. We show that over a range of glass stability, sound damping scales linearly with the fraction of particles in the defects. However, sound is still attenuated in ultra-stable glasses where no defects are identified. We show that sound damping in these glasses is due to nearly uniformly distributed non-affine, microscopic forces that arise after macroscopic deformations of non-centrosymetric structures. To fully understand sound attenuation in glasses one has to consider contributions from defects and a defect-free background, which represents a new paradigm of sound damping in glasses.
title The Origin of Sound Damping in Amorphous Solids: Defects and Beyond
topic Disordered Systems and Neural Networks
Materials Science
url https://arxiv.org/abs/2406.18667