A review on magnetic field induced spin crossover in LaCoO$_{3}$ up to 600 T

Fuente: arXiv
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Auteurs principaux: Ikeda, Akihiko, Matsuda, Yasuhiro H., Sato, Keisuke, Nasu, Joji
Format: Preprint
Publié: 2024
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author Ikeda, Akihiko
Matsuda, Yasuhiro H.
Sato, Keisuke
Nasu, Joji
author_facet Ikeda, Akihiko
Matsuda, Yasuhiro H.
Sato, Keisuke
Nasu, Joji
contents \lco{} is known for its two-step spin crossover as a function of temperature. Despite efforts spanning over half a century, the origin of this phenomenon is still debated, particularly regarding how the microscopic spin states are involved in the observed macroscopic two-step spin crossover. High magnetic field studies on LaCoO$_{3}$ are performed because the magnetic field-induced spin crossover is induced, where the magnetic excited states become more stable in high magnetic fields than the non-magnetic ground states. This review focuses on the findings in LaCoO$_{3}$ at high magnetic fields over the last decade. A complex phase diagram has been revealed at high magnetic fields instead of solving the conventional problem of LaCoO$_{3}$. It suggests that appreciable spin state correlations are in play in LaCoO$_{3}$. The possibility of exciton condensation is also discussed.
format Preprint
id arxiv_https___arxiv_org_abs_2407_00645
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle A review on magnetic field induced spin crossover in LaCoO$_{3}$ up to 600 T
Ikeda, Akihiko
Matsuda, Yasuhiro H.
Sato, Keisuke
Nasu, Joji
Strongly Correlated Electrons
\lco{} is known for its two-step spin crossover as a function of temperature. Despite efforts spanning over half a century, the origin of this phenomenon is still debated, particularly regarding how the microscopic spin states are involved in the observed macroscopic two-step spin crossover. High magnetic field studies on LaCoO$_{3}$ are performed because the magnetic field-induced spin crossover is induced, where the magnetic excited states become more stable in high magnetic fields than the non-magnetic ground states. This review focuses on the findings in LaCoO$_{3}$ at high magnetic fields over the last decade. A complex phase diagram has been revealed at high magnetic fields instead of solving the conventional problem of LaCoO$_{3}$. It suggests that appreciable spin state correlations are in play in LaCoO$_{3}$. The possibility of exciton condensation is also discussed.
title A review on magnetic field induced spin crossover in LaCoO$_{3}$ up to 600 T
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2407.00645