Orbital origin of magnetic moment enhancement induced by charge density wave in kagome FeGe

Fuente: arXiv
Salvato in:
Dettagli Bibliografici
Autori principali: Han, Shulun, Li, Linyang, Tang, Chi Sin, Wang, Qi, Zhang, Lingfeng, Diao, Caozheng, Zhao, Mingwen, Sun, Shuo, Tian, Lijun, Breese, Mark B. H., Cai, Chuanbing, Milosevic, Milorad V., Qi, Yanpeng, Wee, Andrew T. S., Yin, Xinmao
Natura: Preprint
Pubblicazione: 2024
Soggetti:
Accesso online:
Tags: Aggiungi Tag
Nessun Tag, puoi essere il primo ad aggiungerne!!
_version_ 1866929404685320192
author Han, Shulun
Li, Linyang
Tang, Chi Sin
Wang, Qi
Zhang, Lingfeng
Diao, Caozheng
Zhao, Mingwen
Sun, Shuo
Tian, Lijun
Breese, Mark B. H.
Cai, Chuanbing
Milosevic, Milorad V.
Qi, Yanpeng
Wee, Andrew T. S.
Yin, Xinmao
author_facet Han, Shulun
Li, Linyang
Tang, Chi Sin
Wang, Qi
Zhang, Lingfeng
Diao, Caozheng
Zhao, Mingwen
Sun, Shuo
Tian, Lijun
Breese, Mark B. H.
Cai, Chuanbing
Milosevic, Milorad V.
Qi, Yanpeng
Wee, Andrew T. S.
Yin, Xinmao
contents Interactions among various electronic states such as CDW, magnetism, and superconductivity are of high significance in strongly correlated systems. While significant progress has been made in understanding the relationship between CDW and superconductivity, the interplay between CDW and magnetic order remains largely elusive. Kagome lattices, which intertwine nontrivial topology, charge order, and magnetism, offer an ideal platform for such studies. The kagome magnet FeGe, hosting the unique coupling between CDW and magnetism, has recently garnered considerable attention in that respect. Here we reveal the significant role of the orbital coupling effect during the CDW phase transition, highlighting the orbital origin of the magnetic moment enhancement in FeGe. Our X ray absorption experiments and first principles calculations illuminate the temperature dependent behavior of Fe3d_Ge4p orbital hybridization and corroborate its pivotal impact on the magnetic properties of FeGe. These findings introduce an orbital dimension to the correlation between charge and magnetic degrees of freedom, advancing our understanding of the intriguing quantum phases resulting from this interplay.
format Preprint
id arxiv_https___arxiv_org_abs_2407_01076
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Orbital origin of magnetic moment enhancement induced by charge density wave in kagome FeGe
Han, Shulun
Li, Linyang
Tang, Chi Sin
Wang, Qi
Zhang, Lingfeng
Diao, Caozheng
Zhao, Mingwen
Sun, Shuo
Tian, Lijun
Breese, Mark B. H.
Cai, Chuanbing
Milosevic, Milorad V.
Qi, Yanpeng
Wee, Andrew T. S.
Yin, Xinmao
Strongly Correlated Electrons
Interactions among various electronic states such as CDW, magnetism, and superconductivity are of high significance in strongly correlated systems. While significant progress has been made in understanding the relationship between CDW and superconductivity, the interplay between CDW and magnetic order remains largely elusive. Kagome lattices, which intertwine nontrivial topology, charge order, and magnetism, offer an ideal platform for such studies. The kagome magnet FeGe, hosting the unique coupling between CDW and magnetism, has recently garnered considerable attention in that respect. Here we reveal the significant role of the orbital coupling effect during the CDW phase transition, highlighting the orbital origin of the magnetic moment enhancement in FeGe. Our X ray absorption experiments and first principles calculations illuminate the temperature dependent behavior of Fe3d_Ge4p orbital hybridization and corroborate its pivotal impact on the magnetic properties of FeGe. These findings introduce an orbital dimension to the correlation between charge and magnetic degrees of freedom, advancing our understanding of the intriguing quantum phases resulting from this interplay.
title Orbital origin of magnetic moment enhancement induced by charge density wave in kagome FeGe
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2407.01076