Analytical Expression for Continuum-continuum Transition Amplitude of Hydrogen-like Atoms with Angular-momentum Dependence

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Main Authors: Ji, Jia-Bao, Ueda, Kiyoshi, Han, Meng, Wörner, Hans Jakob
Format: Preprint
Published: 2024
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_version_ 1866910645054603264
author Ji, Jia-Bao
Ueda, Kiyoshi
Han, Meng
Wörner, Hans Jakob
author_facet Ji, Jia-Bao
Ueda, Kiyoshi
Han, Meng
Wörner, Hans Jakob
contents Attosecond chronoscopy typically utilises interfering two-photon transitions to access the phase information. Simulating these two-photon transitions is challenging due to the continuum-continuum transition term. The hydrogenic approximation within second-order perturbation theory has been widely used due to the existence of analytical expressions of the wave functions. So far, only (partially) asymptotic results have been derived, which fail to correctly describe the low-kinetic-energy behaviour, especially for high angular-momentum states. Here, we report an analytical expression that overcome these limitations. They are based on the Appell's F1 function and use the confluent hypergeometric function of the second kind as the intermediate states. We show that the derived formula quantitatively agrees with the numerical simulations using the time-dependent Schr{ö}dinger equation for various angular-momentum states, which improves the accuracy compared to the other analytical approaches that were previously reported. Furthermore, we give an angular-momentum-dependent asymptotic form of the outgoing wavefunction and their continuum-continuum dipole transition amplitudes.
format Preprint
id arxiv_https___arxiv_org_abs_2407_09662
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Analytical Expression for Continuum-continuum Transition Amplitude of Hydrogen-like Atoms with Angular-momentum Dependence
Ji, Jia-Bao
Ueda, Kiyoshi
Han, Meng
Wörner, Hans Jakob
Atomic Physics
Mathematical Physics
Attosecond chronoscopy typically utilises interfering two-photon transitions to access the phase information. Simulating these two-photon transitions is challenging due to the continuum-continuum transition term. The hydrogenic approximation within second-order perturbation theory has been widely used due to the existence of analytical expressions of the wave functions. So far, only (partially) asymptotic results have been derived, which fail to correctly describe the low-kinetic-energy behaviour, especially for high angular-momentum states. Here, we report an analytical expression that overcome these limitations. They are based on the Appell's F1 function and use the confluent hypergeometric function of the second kind as the intermediate states. We show that the derived formula quantitatively agrees with the numerical simulations using the time-dependent Schr{ö}dinger equation for various angular-momentum states, which improves the accuracy compared to the other analytical approaches that were previously reported. Furthermore, we give an angular-momentum-dependent asymptotic form of the outgoing wavefunction and their continuum-continuum dipole transition amplitudes.
title Analytical Expression for Continuum-continuum Transition Amplitude of Hydrogen-like Atoms with Angular-momentum Dependence
topic Atomic Physics
Mathematical Physics
url https://arxiv.org/abs/2407.09662