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Main Authors: Sun, Yanwen, Chen, Chaobo, Albert, Thies J., Li, Haoyuan, Arefev, Mikhail I., Chen, Ying, Dunne, Mike, Glownia, James M., Hoffmann, Matthias, Hurley, Matthew J., Mo, Mianzhen, Nguyen, Quynh L., Sato, Takahiro, Song, Sanghoon, Sun, Peihao, Sutton, Mark, Teitelbaum, Samuel, Valavanis, Antonios S., Wang, Nan, Zhu, Diling, Zhigilei, Leonid V., Sokolowski-Tinten, Klaus
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2407.10505
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author Sun, Yanwen
Chen, Chaobo
Albert, Thies J.
Li, Haoyuan
Arefev, Mikhail I.
Chen, Ying
Dunne, Mike
Glownia, James M.
Hoffmann, Matthias
Hurley, Matthew J.
Mo, Mianzhen
Nguyen, Quynh L.
Sato, Takahiro
Song, Sanghoon
Sun, Peihao
Sutton, Mark
Teitelbaum, Samuel
Valavanis, Antonios S.
Wang, Nan
Zhu, Diling
Zhigilei, Leonid V.
Sokolowski-Tinten, Klaus
author_facet Sun, Yanwen
Chen, Chaobo
Albert, Thies J.
Li, Haoyuan
Arefev, Mikhail I.
Chen, Ying
Dunne, Mike
Glownia, James M.
Hoffmann, Matthias
Hurley, Matthew J.
Mo, Mianzhen
Nguyen, Quynh L.
Sato, Takahiro
Song, Sanghoon
Sun, Peihao
Sutton, Mark
Teitelbaum, Samuel
Valavanis, Antonios S.
Wang, Nan
Zhu, Diling
Zhigilei, Leonid V.
Sokolowski-Tinten, Klaus
contents Femtosecond laser ablation is a process that bears both fundamental physics interest and has wide industrial applications. For decades, the lack of probes on the relevant time and length scales has prevented access to the highly nonequilibrium phase decomposition processes triggered by laser excitation. Enabled by the unprecedented intense femtosecond X-ray pulses delivered by an X-ray free electron laser, we report here results of time-resolved small angle scattering measurements on the dynamics of nanoscale phase decomposition in thin gold films upon femtosecond laser-induced ablation. By analyzing the features imprinted onto the small angle diffraction patterns, the transient heterogeneous density distributions within the ablation plume as obtained from molecular dynamics simulations get direct experimental confirmation.
format Preprint
id arxiv_https___arxiv_org_abs_2407_10505
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Dynamics of Nanoscale Phase Decomposition in Laser Ablation
Sun, Yanwen
Chen, Chaobo
Albert, Thies J.
Li, Haoyuan
Arefev, Mikhail I.
Chen, Ying
Dunne, Mike
Glownia, James M.
Hoffmann, Matthias
Hurley, Matthew J.
Mo, Mianzhen
Nguyen, Quynh L.
Sato, Takahiro
Song, Sanghoon
Sun, Peihao
Sutton, Mark
Teitelbaum, Samuel
Valavanis, Antonios S.
Wang, Nan
Zhu, Diling
Zhigilei, Leonid V.
Sokolowski-Tinten, Klaus
Materials Science
Femtosecond laser ablation is a process that bears both fundamental physics interest and has wide industrial applications. For decades, the lack of probes on the relevant time and length scales has prevented access to the highly nonequilibrium phase decomposition processes triggered by laser excitation. Enabled by the unprecedented intense femtosecond X-ray pulses delivered by an X-ray free electron laser, we report here results of time-resolved small angle scattering measurements on the dynamics of nanoscale phase decomposition in thin gold films upon femtosecond laser-induced ablation. By analyzing the features imprinted onto the small angle diffraction patterns, the transient heterogeneous density distributions within the ablation plume as obtained from molecular dynamics simulations get direct experimental confirmation.
title Dynamics of Nanoscale Phase Decomposition in Laser Ablation
topic Materials Science
url https://arxiv.org/abs/2407.10505