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Main Authors: Kavand, Marzieh, Phillips, Zoe, Koll, William H., Hamilton, Morgan, Perez-Hoyos, Ethel, Greer, Rianna, Ara, Ferdous, Pharis, Daniel, Maleki, Kian, Xu, Mingyu, Taniguchi, Takashi, Canfield, Paul, Flatté, Michael E., Freedman, Danna E., Gupta, Jay, Johnston-Halperin, Ezekiel
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2407.11189
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author Kavand, Marzieh
Phillips, Zoe
Koll, William H.
Hamilton, Morgan
Perez-Hoyos, Ethel
Greer, Rianna
Ara, Ferdous
Pharis, Daniel
Maleki, Kian
Xu, Mingyu
Taniguchi, Takashi
Canfield, Paul
Flatté, Michael E.
Freedman, Danna E.
Gupta, Jay
Johnston-Halperin, Ezekiel
author_facet Kavand, Marzieh
Phillips, Zoe
Koll, William H.
Hamilton, Morgan
Perez-Hoyos, Ethel
Greer, Rianna
Ara, Ferdous
Pharis, Daniel
Maleki, Kian
Xu, Mingyu
Taniguchi, Takashi
Canfield, Paul
Flatté, Michael E.
Freedman, Danna E.
Gupta, Jay
Johnston-Halperin, Ezekiel
contents Here, we present an all-electrical readout mechanism for quasi-0D quantum states (0D-QS) such as point defects, adatoms and molecules, that is modular and general, providing an approach that is amenable to scaling and integration with other solid-state quantum technologies. Our approach relies on the crea-tion of high-quality tunnel junctions via the mechanical exfoliation and stacking of multi-layer gra-phene (MLG) and hexagonal boron nitride (hBN) to encapsulate the target system in an MLG/hBN/0D-QS/hBN/MLG heterostructure. This structure allows for all-electronic spectroscopy and readout of candidate systems through a combination of coulomb and spin-blockade. As a proof of principle, we demonstrate electronic tunneling spectroscopy of point defects in hBN and the molecular qubit vanadyl phthalocyanine (VOPc). Our approach demonstrates a new pathway for the incorporation of molecules and atomic defects into solid-state quantum devices and circuits along with a readout scheme that does not rely on highly-constrained optical processes for photonic readout.
format Preprint
id arxiv_https___arxiv_org_abs_2407_11189
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle A general and modular approach to solid-state integration and readout of zero-dimensional quantum systems
Kavand, Marzieh
Phillips, Zoe
Koll, William H.
Hamilton, Morgan
Perez-Hoyos, Ethel
Greer, Rianna
Ara, Ferdous
Pharis, Daniel
Maleki, Kian
Xu, Mingyu
Taniguchi, Takashi
Canfield, Paul
Flatté, Michael E.
Freedman, Danna E.
Gupta, Jay
Johnston-Halperin, Ezekiel
Materials Science
Here, we present an all-electrical readout mechanism for quasi-0D quantum states (0D-QS) such as point defects, adatoms and molecules, that is modular and general, providing an approach that is amenable to scaling and integration with other solid-state quantum technologies. Our approach relies on the crea-tion of high-quality tunnel junctions via the mechanical exfoliation and stacking of multi-layer gra-phene (MLG) and hexagonal boron nitride (hBN) to encapsulate the target system in an MLG/hBN/0D-QS/hBN/MLG heterostructure. This structure allows for all-electronic spectroscopy and readout of candidate systems through a combination of coulomb and spin-blockade. As a proof of principle, we demonstrate electronic tunneling spectroscopy of point defects in hBN and the molecular qubit vanadyl phthalocyanine (VOPc). Our approach demonstrates a new pathway for the incorporation of molecules and atomic defects into solid-state quantum devices and circuits along with a readout scheme that does not rely on highly-constrained optical processes for photonic readout.
title A general and modular approach to solid-state integration and readout of zero-dimensional quantum systems
topic Materials Science
url https://arxiv.org/abs/2407.11189