Fate of transient order parameter domain walls in ultrafast experiments

Fuente: arXiv
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Main Authors: Kong, Lingxian, Shindou, Ryuichi, Sun, Zhiyuan
Format: Preprint
Published: 2024
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author Kong, Lingxian
Shindou, Ryuichi
Sun, Zhiyuan
author_facet Kong, Lingxian
Shindou, Ryuichi
Sun, Zhiyuan
contents In ultrafast experiments, an optical pump pulse often generates transient domain walls of the order parameter in materials with spontaneous symmetry breaking, due to either a finite penetration depth of light on a three-dimensional (3D) material, or a finite spot size on a two-dimensional (2D) material. We show that the domain wall decays due to unstable order parameter fluctuations. We study a generic system with $U(1)$-symmetric order, and those with an additional weak $Z_2$ ($U(1)$-symmetry-breaking) term, representing the charge-density-wave (CDW) orders in recent experiments. During the first stage of the decay dynamics, exponentially growing thermal fluctuations convert the domain wall into an interface with randomly distributed topological defects. In the second stage, the topological defects undergo a coarsening dynamics within the interface. For a 2D interface in a 3D system, the coarsening dynamics leads to a diffusive growth of the correlation length. For a one-dimensional (1D) interface in a 2D system with the weak $Z_2$ term, the correlation-length growth shows a crossover from diffusive to sub-diffusive behavior.
format Preprint
id arxiv_https___arxiv_org_abs_2407_14250
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Fate of transient order parameter domain walls in ultrafast experiments
Kong, Lingxian
Shindou, Ryuichi
Sun, Zhiyuan
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Statistical Mechanics
In ultrafast experiments, an optical pump pulse often generates transient domain walls of the order parameter in materials with spontaneous symmetry breaking, due to either a finite penetration depth of light on a three-dimensional (3D) material, or a finite spot size on a two-dimensional (2D) material. We show that the domain wall decays due to unstable order parameter fluctuations. We study a generic system with $U(1)$-symmetric order, and those with an additional weak $Z_2$ ($U(1)$-symmetry-breaking) term, representing the charge-density-wave (CDW) orders in recent experiments. During the first stage of the decay dynamics, exponentially growing thermal fluctuations convert the domain wall into an interface with randomly distributed topological defects. In the second stage, the topological defects undergo a coarsening dynamics within the interface. For a 2D interface in a 3D system, the coarsening dynamics leads to a diffusive growth of the correlation length. For a one-dimensional (1D) interface in a 2D system with the weak $Z_2$ term, the correlation-length growth shows a crossover from diffusive to sub-diffusive behavior.
title Fate of transient order parameter domain walls in ultrafast experiments
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Statistical Mechanics
url https://arxiv.org/abs/2407.14250