Structural Relaxation in Simple Yield Stress Materials Influences Their Rheology

Fuente: arXiv
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Auteurs principaux: Farain, Kasra, Bonn, Daniel
Format: Preprint
Publié: 2024
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author Farain, Kasra
Bonn, Daniel
author_facet Farain, Kasra
Bonn, Daniel
contents Simple yield stress materials are composed of soft particles, bubbles, or droplets with purely repulsive forces. The constituent elements are typically too large to undergo thermal fluctuations, suggesting that the internal structure of the material, and therefore the rheology, should not change over time. We explore the rheology of Carbopol, a prototypical simple yield stress material, and show that gradual structural relaxation of the material results in a small yet significant reduction in the dynamic yield stress. This relaxation process can lead to a non-monotonic creep deformation rate under constant stress, culminating in delayed fluidization of the material. These findings show that the yield stress is not merely a static material property but may be a function of the internal structure of the material.
format Preprint
id arxiv_https___arxiv_org_abs_2407_16619
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Structural Relaxation in Simple Yield Stress Materials Influences Their Rheology
Farain, Kasra
Bonn, Daniel
Soft Condensed Matter
Materials Science
Simple yield stress materials are composed of soft particles, bubbles, or droplets with purely repulsive forces. The constituent elements are typically too large to undergo thermal fluctuations, suggesting that the internal structure of the material, and therefore the rheology, should not change over time. We explore the rheology of Carbopol, a prototypical simple yield stress material, and show that gradual structural relaxation of the material results in a small yet significant reduction in the dynamic yield stress. This relaxation process can lead to a non-monotonic creep deformation rate under constant stress, culminating in delayed fluidization of the material. These findings show that the yield stress is not merely a static material property but may be a function of the internal structure of the material.
title Structural Relaxation in Simple Yield Stress Materials Influences Their Rheology
topic Soft Condensed Matter
Materials Science
url https://arxiv.org/abs/2407.16619