Unveiling van Hove singularity modulation and fluctuated charge order in kagome superconductor $\rm{CsV_3Sb_5}$ via time-resolved ARPES

Fuente: arXiv
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Main Authors: Zhong, Yigui, Suzuki, Takeshi, Liu, Hongxiong, Liu, Kecheng, Nie, Zhengwei, Shi, Youguo, Meng, Sheng, Lv, Baiqing, Ding, Hong, Kanai, Teruto, Itatani, Jiro, Shin, Shik, Okazaki, Kozo
Format: Preprint
Published: 2024
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author Zhong, Yigui
Suzuki, Takeshi
Liu, Hongxiong
Liu, Kecheng
Nie, Zhengwei
Shi, Youguo
Meng, Sheng
Lv, Baiqing
Ding, Hong
Kanai, Teruto
Itatani, Jiro
Shin, Shik
Okazaki, Kozo
author_facet Zhong, Yigui
Suzuki, Takeshi
Liu, Hongxiong
Liu, Kecheng
Nie, Zhengwei
Shi, Youguo
Meng, Sheng
Lv, Baiqing
Ding, Hong
Kanai, Teruto
Itatani, Jiro
Shin, Shik
Okazaki, Kozo
contents Kagome superconductor CsV3Sb5, which exhibits intertwined unconventional charge density wave (CDW) and superconductivity, has garnered significant attention recently. Despite extensive static studies, the nature of these exotic electronic orders remains elusive. In this study, we investigate the non-equilibrium electronic structure of CsV3Sb5 via time- and angle-resolved photoemission spectroscopy. Our results reveal that upon laser excitation, the van Hove singularities immediately shift towards the Fermi level and subsequently oscillate in sync with a 1.3 THz coherent phonon mode. By analyzing the coherent intensity oscillations in the energy-momentum (E-k) map, we find that this coherent phonon is strongly coupled with electronic bands from both Sb and V orbitals. While typically observable only in the CDW state, remarkably, we find that the 1.3-THz coherent phonon mode can be persistently excited at temperatures above T_CDW, suggesting the potential existence of fluctuated CDW in CsV3Sb5. These findings enhance our understanding of the unconventional CDW control of kagome superconductivity.
format Preprint
id arxiv_https___arxiv_org_abs_2407_17015
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Unveiling van Hove singularity modulation and fluctuated charge order in kagome superconductor $\rm{CsV_3Sb_5}$ via time-resolved ARPES
Zhong, Yigui
Suzuki, Takeshi
Liu, Hongxiong
Liu, Kecheng
Nie, Zhengwei
Shi, Youguo
Meng, Sheng
Lv, Baiqing
Ding, Hong
Kanai, Teruto
Itatani, Jiro
Shin, Shik
Okazaki, Kozo
Materials Science
Strongly Correlated Electrons
Superconductivity
Kagome superconductor CsV3Sb5, which exhibits intertwined unconventional charge density wave (CDW) and superconductivity, has garnered significant attention recently. Despite extensive static studies, the nature of these exotic electronic orders remains elusive. In this study, we investigate the non-equilibrium electronic structure of CsV3Sb5 via time- and angle-resolved photoemission spectroscopy. Our results reveal that upon laser excitation, the van Hove singularities immediately shift towards the Fermi level and subsequently oscillate in sync with a 1.3 THz coherent phonon mode. By analyzing the coherent intensity oscillations in the energy-momentum (E-k) map, we find that this coherent phonon is strongly coupled with electronic bands from both Sb and V orbitals. While typically observable only in the CDW state, remarkably, we find that the 1.3-THz coherent phonon mode can be persistently excited at temperatures above T_CDW, suggesting the potential existence of fluctuated CDW in CsV3Sb5. These findings enhance our understanding of the unconventional CDW control of kagome superconductivity.
title Unveiling van Hove singularity modulation and fluctuated charge order in kagome superconductor $\rm{CsV_3Sb_5}$ via time-resolved ARPES
topic Materials Science
Strongly Correlated Electrons
Superconductivity
url https://arxiv.org/abs/2407.17015