The incredible diversity of structural and magnetic instabilities in EuTiO3: from paramagnetic to spin glass, spin liquid and antiferromagnetic order

Fuente: arXiv
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Main Authors: Bussmann-Holder, Annette, Kremer, Reinhard K., Liarokapis, Efthymios, Roleder, Krystian
Format: Preprint
Published: 2024
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author Bussmann-Holder, Annette
Kremer, Reinhard K.
Liarokapis, Efthymios
Roleder, Krystian
author_facet Bussmann-Holder, Annette
Kremer, Reinhard K.
Liarokapis, Efthymios
Roleder, Krystian
contents The perovskite oxide EuTiO3 (ETO) has attracted increased scientific interest due to its potential multiferroic properties and magnetic activity above and below its structural phase transition at TS=282K. Various experiments have indirectly evidenced that this transition is neither a cubic tetragonal nor the only one occurring in ETO. Here, we show new results demonstrating two further instabilities below TS based on lattice dynamics and spin-phonon interactions combined with a Landau free energy model with coupled order parameters. The new transition temperatures perfectly agree with available experimental data where further instabilities have been anticipated.
format Preprint
id arxiv_https___arxiv_org_abs_2407_17878
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle The incredible diversity of structural and magnetic instabilities in EuTiO3: from paramagnetic to spin glass, spin liquid and antiferromagnetic order
Bussmann-Holder, Annette
Kremer, Reinhard K.
Liarokapis, Efthymios
Roleder, Krystian
Materials Science
The perovskite oxide EuTiO3 (ETO) has attracted increased scientific interest due to its potential multiferroic properties and magnetic activity above and below its structural phase transition at TS=282K. Various experiments have indirectly evidenced that this transition is neither a cubic tetragonal nor the only one occurring in ETO. Here, we show new results demonstrating two further instabilities below TS based on lattice dynamics and spin-phonon interactions combined with a Landau free energy model with coupled order parameters. The new transition temperatures perfectly agree with available experimental data where further instabilities have been anticipated.
title The incredible diversity of structural and magnetic instabilities in EuTiO3: from paramagnetic to spin glass, spin liquid and antiferromagnetic order
topic Materials Science
url https://arxiv.org/abs/2407.17878