Large Nernst Effect in a layered metallic antiferromagnet EuAl$_2$Si$_2$

Fuente: arXiv
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Main Authors: Yang, Kunya, Xia, Wei, Mi, Xinrun, zhang, Yiyue, zhang, Long, Wang, Aifeng, Chai, Yisheng, Zhou, Xiaoyuan, Guo, Yanfeng, He, Mingquan
Format: Preprint
Published: 2024
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_version_ 1866910664668217344
author Yang, Kunya
Xia, Wei
Mi, Xinrun
zhang, Yiyue
zhang, Long
Wang, Aifeng
Chai, Yisheng
Zhou, Xiaoyuan
Guo, Yanfeng
He, Mingquan
author_facet Yang, Kunya
Xia, Wei
Mi, Xinrun
zhang, Yiyue
zhang, Long
Wang, Aifeng
Chai, Yisheng
Zhou, Xiaoyuan
Guo, Yanfeng
He, Mingquan
contents The large Nernst effect is advantageous for developing transverse Nernst thermoelectric generators or Ettingshausen coolers within a single component, avoiding the complexity of electron- and hole-modules in longitudinal Seebeck thermoelectric devices. We report a large Nernst signal reaching 130 uV/K at 8 K and 13 T in the layered metallic antiferromagnet EuAl$_2$Si$_2$. Notably, this large transverse Nernst thermopower is two orders of magnitude greater than its longitudinal counterpart. The Nernst coefficient peaks around 4 K and 8 K at 3 T and 13 T, respectively. At similar temperatures, both the Hall coefficient and the Seebeck signal change sign. Additionally, nearly compensated electron- and hole-like carriers with high mobility ($\sim$ 4000 cm$^2$/Vs at 4 K) are revealed from the magnetoconductivity. These findings suggest that the large Nernst effect and vanishing Seebeck thermopower in EuAl$_2$Si$_2$ are due to the compensated electron- and hole-like bands, along with the high mobility of the Weyl band near the Fermi level. Our results underscore the importance of band compensation and topological fermiology in achieving large Nernst thermopower and exploring potential Nernst thermoelectric applications at low temperatures.
format Preprint
id arxiv_https___arxiv_org_abs_2407_18460
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Large Nernst Effect in a layered metallic antiferromagnet EuAl$_2$Si$_2$
Yang, Kunya
Xia, Wei
Mi, Xinrun
zhang, Yiyue
zhang, Long
Wang, Aifeng
Chai, Yisheng
Zhou, Xiaoyuan
Guo, Yanfeng
He, Mingquan
Materials Science
Strongly Correlated Electrons
The large Nernst effect is advantageous for developing transverse Nernst thermoelectric generators or Ettingshausen coolers within a single component, avoiding the complexity of electron- and hole-modules in longitudinal Seebeck thermoelectric devices. We report a large Nernst signal reaching 130 uV/K at 8 K and 13 T in the layered metallic antiferromagnet EuAl$_2$Si$_2$. Notably, this large transverse Nernst thermopower is two orders of magnitude greater than its longitudinal counterpart. The Nernst coefficient peaks around 4 K and 8 K at 3 T and 13 T, respectively. At similar temperatures, both the Hall coefficient and the Seebeck signal change sign. Additionally, nearly compensated electron- and hole-like carriers with high mobility ($\sim$ 4000 cm$^2$/Vs at 4 K) are revealed from the magnetoconductivity. These findings suggest that the large Nernst effect and vanishing Seebeck thermopower in EuAl$_2$Si$_2$ are due to the compensated electron- and hole-like bands, along with the high mobility of the Weyl band near the Fermi level. Our results underscore the importance of band compensation and topological fermiology in achieving large Nernst thermopower and exploring potential Nernst thermoelectric applications at low temperatures.
title Large Nernst Effect in a layered metallic antiferromagnet EuAl$_2$Si$_2$
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2407.18460