Topological Phase Transition in Quasi-One-Dimensional Bismuth Iodide Bi4I4

Fuente: arXiv
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Autori principali: Zhao, W. X., Yang, M., Du, X., Li, Y. D., Zhai, K. Y., Hu, Y. Q., Han, J. F., Huang, Y., Liu, Z. K., Yao, Y. G., Zhuang, J. C., Du, Y., Zhou, J. J., Chen, Y. L., Yang, L. X.
Natura: Preprint
Pubblicazione: 2024
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author Zhao, W. X.
Yang, M.
Du, X.
Li, Y. D.
Zhai, K. Y.
Hu, Y. Q.
Han, J. F.
Huang, Y.
Liu, Z. K.
Yao, Y. G.
Zhuang, J. C.
Du, Y.
Zhou, J. J.
Chen, Y. L.
Yang, L. X.
author_facet Zhao, W. X.
Yang, M.
Du, X.
Li, Y. D.
Zhai, K. Y.
Hu, Y. Q.
Han, J. F.
Huang, Y.
Liu, Z. K.
Yao, Y. G.
Zhuang, J. C.
Du, Y.
Zhou, J. J.
Chen, Y. L.
Yang, L. X.
contents The exploration of topological quantum materials and topological phase transitions is at the forefront of modern condensed matter physics. Quasi-one-dimensional (quasi-1D) bismuth iodide Bi4I4 exhibits versatile topological phases of matter including weak topological insulator (WTI) and higher-order topological insulator (HOTI) phases with high tunability in response to external parameters. In this work, performing laser-based angle-resolved photoemission spectroscopy with submicron spatial resolution (micro-ARPES), we comprehensively investigate the fine electronic structure and topological phase transition of Bi4I4. Our examination of the low-temperature α-phase reveals the presence of an energy gap on the (100) surface, providing spectroscopic evidence for the HOTI phase. Conversely, the high-temperature β-Bi4I4 harbors a gapless Dirac fermion on the (100) surface alongside gapped states on the (001) surface, thereby establishing a WTI phase. By tracking the temperature evolution of the (100) surface states, we unveil a thermal hysteresis of the surface gap in line with the α-β structural phase transition. Our findings elucidate the topological properties of Bi4I4 and directly evidence a temperature-induced topological phase transition from WTI to HOTI, which paves the way to potential applications based on the room-temperature topological phase transition in the quasi-1D topological quantum material.
format Preprint
id arxiv_https___arxiv_org_abs_2407_19375
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Topological Phase Transition in Quasi-One-Dimensional Bismuth Iodide Bi4I4
Zhao, W. X.
Yang, M.
Du, X.
Li, Y. D.
Zhai, K. Y.
Hu, Y. Q.
Han, J. F.
Huang, Y.
Liu, Z. K.
Yao, Y. G.
Zhuang, J. C.
Du, Y.
Zhou, J. J.
Chen, Y. L.
Yang, L. X.
Materials Science
Mesoscale and Nanoscale Physics
The exploration of topological quantum materials and topological phase transitions is at the forefront of modern condensed matter physics. Quasi-one-dimensional (quasi-1D) bismuth iodide Bi4I4 exhibits versatile topological phases of matter including weak topological insulator (WTI) and higher-order topological insulator (HOTI) phases with high tunability in response to external parameters. In this work, performing laser-based angle-resolved photoemission spectroscopy with submicron spatial resolution (micro-ARPES), we comprehensively investigate the fine electronic structure and topological phase transition of Bi4I4. Our examination of the low-temperature α-phase reveals the presence of an energy gap on the (100) surface, providing spectroscopic evidence for the HOTI phase. Conversely, the high-temperature β-Bi4I4 harbors a gapless Dirac fermion on the (100) surface alongside gapped states on the (001) surface, thereby establishing a WTI phase. By tracking the temperature evolution of the (100) surface states, we unveil a thermal hysteresis of the surface gap in line with the α-β structural phase transition. Our findings elucidate the topological properties of Bi4I4 and directly evidence a temperature-induced topological phase transition from WTI to HOTI, which paves the way to potential applications based on the room-temperature topological phase transition in the quasi-1D topological quantum material.
title Topological Phase Transition in Quasi-One-Dimensional Bismuth Iodide Bi4I4
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2407.19375