The submonolayer assembly of C60F48 surface acceptors on the hydrogen-terminated (100) diamond surface

Fuente: arXiv
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Auteurs principaux: Schenk, Alex K., Rietwyk, Kevin J., Edmonds, Mark T., Tadich, Anton, Pakes, Chris I.
Format: Preprint
Publié: 2024
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author Schenk, Alex K.
Rietwyk, Kevin J.
Edmonds, Mark T.
Tadich, Anton
Pakes, Chris I.
author_facet Schenk, Alex K.
Rietwyk, Kevin J.
Edmonds, Mark T.
Tadich, Anton
Pakes, Chris I.
contents We have characterised the submonolayer assembly of C60F48 molecular surface acceptors on the hydrogen terminated (100) diamond surface using scanning tunneling microscopy and X-ray photoelectron spectroscopy, and explored the influence this assembly has on the energy level alignment which governs surface transfer doping. Following deposition, disordered multilayered islands are observed. Annealing to 90$^{\circ} \rm{C}$ causes a transition from dewetting multi-layered islands to a single wetting layer at sufficiently high coverage, accompanied by a change in the energy alignment between the C60F48 and the diamond surface which consequently decreased the carrier density induced by transfer doping by 20%.
format Preprint
id arxiv_https___arxiv_org_abs_2407_19649
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle The submonolayer assembly of C60F48 surface acceptors on the hydrogen-terminated (100) diamond surface
Schenk, Alex K.
Rietwyk, Kevin J.
Edmonds, Mark T.
Tadich, Anton
Pakes, Chris I.
Materials Science
We have characterised the submonolayer assembly of C60F48 molecular surface acceptors on the hydrogen terminated (100) diamond surface using scanning tunneling microscopy and X-ray photoelectron spectroscopy, and explored the influence this assembly has on the energy level alignment which governs surface transfer doping. Following deposition, disordered multilayered islands are observed. Annealing to 90$^{\circ} \rm{C}$ causes a transition from dewetting multi-layered islands to a single wetting layer at sufficiently high coverage, accompanied by a change in the energy alignment between the C60F48 and the diamond surface which consequently decreased the carrier density induced by transfer doping by 20%.
title The submonolayer assembly of C60F48 surface acceptors on the hydrogen-terminated (100) diamond surface
topic Materials Science
url https://arxiv.org/abs/2407.19649