Evidence for Two-dimensional Weyl Fermions in Air-Stable Monolayer PtTe$_{1.75}$

Fuente: arXiv
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Autori principali: Cai, Zhihao, Cao, Haijun, Sheng, Haohao, Hu, Xuegao, Sun, Zhenyu, Zhao, Qiaoxiao, Gao, Jisong, Ideta, Shin-ichiro, Shimada, Kenya, Huang, Jiawei, Cheng, Peng, Chen, Lan, Yao, Yugui, Meng, Sheng, Wu, Kehui, Wang, Zhijun, Feng, Baojie
Natura: Preprint
Pubblicazione: 2024
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author Cai, Zhihao
Cao, Haijun
Sheng, Haohao
Hu, Xuegao
Sun, Zhenyu
Zhao, Qiaoxiao
Gao, Jisong
Ideta, Shin-ichiro
Shimada, Kenya
Huang, Jiawei
Cheng, Peng
Chen, Lan
Yao, Yugui
Meng, Sheng
Wu, Kehui
Wang, Zhijun
Feng, Baojie
author_facet Cai, Zhihao
Cao, Haijun
Sheng, Haohao
Hu, Xuegao
Sun, Zhenyu
Zhao, Qiaoxiao
Gao, Jisong
Ideta, Shin-ichiro
Shimada, Kenya
Huang, Jiawei
Cheng, Peng
Chen, Lan
Yao, Yugui
Meng, Sheng
Wu, Kehui
Wang, Zhijun
Feng, Baojie
contents The Weyl semimetals represent a distinct category of topological materials wherein the low-energy excitations appear as the long-sought Weyl fermions. Exotic transport and optical properties are expected because of the chiral anomaly and linear energy-momentum dispersion. While three-dimensional Weyl semimetals have been successfully realized, the quest for their two-dimensional (2D) counterparts is ongoing. Here, we report the realization of 2D Weyl fermions in monolayer PtTe$_{1.75}$, which has strong spin-orbit coupling and lacks inversion symmetry, by combined angle-resolved photoemission spectroscopy, scanning tunneling microscopy, second harmonic generation, X-ray photoelectron spectroscopy measurements, and first-principles calculations. The giant Rashba splitting and band inversion lead to the emergence of three pairs of critical Weyl cones. Moreover, monolayer PtTe$_{1.75}$ exhibits excellent chemical stability in ambient conditions, which is critical for future device applications. The discovery of 2D Weyl fermions in monolayer PtTe$_{1.75}$ opens up new possibilities for designing and fabricating novel spintronic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2407_20606
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Evidence for Two-dimensional Weyl Fermions in Air-Stable Monolayer PtTe$_{1.75}$
Cai, Zhihao
Cao, Haijun
Sheng, Haohao
Hu, Xuegao
Sun, Zhenyu
Zhao, Qiaoxiao
Gao, Jisong
Ideta, Shin-ichiro
Shimada, Kenya
Huang, Jiawei
Cheng, Peng
Chen, Lan
Yao, Yugui
Meng, Sheng
Wu, Kehui
Wang, Zhijun
Feng, Baojie
Mesoscale and Nanoscale Physics
Materials Science
The Weyl semimetals represent a distinct category of topological materials wherein the low-energy excitations appear as the long-sought Weyl fermions. Exotic transport and optical properties are expected because of the chiral anomaly and linear energy-momentum dispersion. While three-dimensional Weyl semimetals have been successfully realized, the quest for their two-dimensional (2D) counterparts is ongoing. Here, we report the realization of 2D Weyl fermions in monolayer PtTe$_{1.75}$, which has strong spin-orbit coupling and lacks inversion symmetry, by combined angle-resolved photoemission spectroscopy, scanning tunneling microscopy, second harmonic generation, X-ray photoelectron spectroscopy measurements, and first-principles calculations. The giant Rashba splitting and band inversion lead to the emergence of three pairs of critical Weyl cones. Moreover, monolayer PtTe$_{1.75}$ exhibits excellent chemical stability in ambient conditions, which is critical for future device applications. The discovery of 2D Weyl fermions in monolayer PtTe$_{1.75}$ opens up new possibilities for designing and fabricating novel spintronic devices.
title Evidence for Two-dimensional Weyl Fermions in Air-Stable Monolayer PtTe$_{1.75}$
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2407.20606