Quantum-metric-induced giant and reversible nonreciprocal transport phenomena in chiral loop-current phases of kagome metals

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Auteurs principaux: Tazai, Rina, Yamakawa, Youichi, Morimoto, Takahiro, Kontani, Hiroshi
Format: Preprint
Publié: 2024
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author Tazai, Rina
Yamakawa, Youichi
Morimoto, Takahiro
Kontani, Hiroshi
author_facet Tazai, Rina
Yamakawa, Youichi
Morimoto, Takahiro
Kontani, Hiroshi
contents Rich spontaneous symmetry-breaking phenomena with nontrivial quantum geometric properties in metals represent central issues in condensed matter physics. In this context, the emergence of chiral loop-current order, accompanied by time-reversal symmetry-symmetry breaking in various kagome metals, has garnered significant attention. Particularly noteworthy is the giant electrical magnetochiral anisotropy (eMChA) in CsV3Sb5, which provides compelling evidence of time-reversal-symmetry and inversion-symmetry breakings. However, the underlying essence of this observation has remained obscured due to the lack of theoretical understanding. Here, we reveal that the loop-current order causes giant and reversible eMChA coefficient, $γ_{eM}$, is proportional to the loop-current-induced orbital magnetization $M_{orb}$ times the lifetime of conduction electrons $τ$. In kagome metals, the derived $γ_{eM}$ is substantial and reversible by minute magnetic fields, due to the large $τ(\gg a_0/v_{Fermi})$ and the field-induced reversal of $M_{orb}$. By considering the experimentally observed stripe charge-density wave, the loop-current state becomes non-centrosymmetric, thereby giving rise to the eMChA. Surprisingly, the quantum-metric, which defines a fundamental geometric aspect of Bloch wavefunctions, acquires significant momentum dependence in the loop-current phase, resulting in a dramatic enhancement of eMChA by $\sim100$ times. This research not only clarifies the fundamental symmetry-breaking states in kagome metals, but also opens a new path for exploring quantum-metric-induced phenomena arising from exotic quantum phase transitions in strongly correlated metals
format Preprint
id arxiv_https___arxiv_org_abs_2408_04233
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Quantum-metric-induced giant and reversible nonreciprocal transport phenomena in chiral loop-current phases of kagome metals
Tazai, Rina
Yamakawa, Youichi
Morimoto, Takahiro
Kontani, Hiroshi
Strongly Correlated Electrons
Superconductivity
Rich spontaneous symmetry-breaking phenomena with nontrivial quantum geometric properties in metals represent central issues in condensed matter physics. In this context, the emergence of chiral loop-current order, accompanied by time-reversal symmetry-symmetry breaking in various kagome metals, has garnered significant attention. Particularly noteworthy is the giant electrical magnetochiral anisotropy (eMChA) in CsV3Sb5, which provides compelling evidence of time-reversal-symmetry and inversion-symmetry breakings. However, the underlying essence of this observation has remained obscured due to the lack of theoretical understanding. Here, we reveal that the loop-current order causes giant and reversible eMChA coefficient, $γ_{eM}$, is proportional to the loop-current-induced orbital magnetization $M_{orb}$ times the lifetime of conduction electrons $τ$. In kagome metals, the derived $γ_{eM}$ is substantial and reversible by minute magnetic fields, due to the large $τ(\gg a_0/v_{Fermi})$ and the field-induced reversal of $M_{orb}$. By considering the experimentally observed stripe charge-density wave, the loop-current state becomes non-centrosymmetric, thereby giving rise to the eMChA. Surprisingly, the quantum-metric, which defines a fundamental geometric aspect of Bloch wavefunctions, acquires significant momentum dependence in the loop-current phase, resulting in a dramatic enhancement of eMChA by $\sim100$ times. This research not only clarifies the fundamental symmetry-breaking states in kagome metals, but also opens a new path for exploring quantum-metric-induced phenomena arising from exotic quantum phase transitions in strongly correlated metals
title Quantum-metric-induced giant and reversible nonreciprocal transport phenomena in chiral loop-current phases of kagome metals
topic Strongly Correlated Electrons
Superconductivity
url https://arxiv.org/abs/2408.04233