Emergent superconductivity and pair density wave at antiphase boundaries of charge density wave order in kagome metals

Fuente: arXiv
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Autori principali: Han, Xianghe, Chen, Hui, Tan, Hengxin, Cao, Zhongyi, Huang, Zihao, Ye, Yuhan, Zhao, Zhen, Shen, Chengmin, Yang, Haitao, Yan, Binghai, Wang, Ziqiang, Gao, Hong-Jun
Natura: Preprint
Pubblicazione: 2024
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author Han, Xianghe
Chen, Hui
Tan, Hengxin
Cao, Zhongyi
Huang, Zihao
Ye, Yuhan
Zhao, Zhen
Shen, Chengmin
Yang, Haitao
Yan, Binghai
Wang, Ziqiang
Gao, Hong-Jun
author_facet Han, Xianghe
Chen, Hui
Tan, Hengxin
Cao, Zhongyi
Huang, Zihao
Ye, Yuhan
Zhao, Zhen
Shen, Chengmin
Yang, Haitao
Yan, Binghai
Wang, Ziqiang
Gao, Hong-Jun
contents Central to the layered kagome lattice superconductors AV3Sb5 (A = K, Cs, Rb) is a cascade of novel quantum states triggered by an unconventional charge density wave (CDW) order. The three-dimensional (3D) order involves a 2x2x2 phase coherent stacking of 2x2 charge density modulations in the kagome plane at low temperatures, exhibiting a CDW energy gap and evidence for time-reversal symmetry breaking. Here we report the discovery of emergent superconductivity and primary pair density wave (PDW) at the antiphase boundaries and stacking faults of bulk CDW order. We find that the π-phase shift dislocations can naturally appear on the surface as the Cs atoms form 2x2 superstructures that are out of phase with the bulk CDW. An incipient narrow band of surface states inside bulk CDW gap emerge close to the Fermi level where a particle-hole symmetric energy gap develops. We demonstrate that the energy gap originates from a novel quasi-2D kagome superconducting state (Tc ~ 5.4 K) intertwined with bulk CDW order, exhibiting an unprecedented vortex core spectrum and spatial modulations of the superconducting gap consistent with a 4x4 PDW. Intriguingly, the 2D kagome superconductivity is shown to be tunable on and off by atomically manipulating the Cs atoms on the surface. Our findings provide fresh new insights for understanding the interplay between the unconventional CDW and superconductivity in kagome metals and a pathway for atomic manipulation and topological defects engineering of quantum many-body states in correlated materials.
format Preprint
id arxiv_https___arxiv_org_abs_2408_06174
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Emergent superconductivity and pair density wave at antiphase boundaries of charge density wave order in kagome metals
Han, Xianghe
Chen, Hui
Tan, Hengxin
Cao, Zhongyi
Huang, Zihao
Ye, Yuhan
Zhao, Zhen
Shen, Chengmin
Yang, Haitao
Yan, Binghai
Wang, Ziqiang
Gao, Hong-Jun
Superconductivity
Central to the layered kagome lattice superconductors AV3Sb5 (A = K, Cs, Rb) is a cascade of novel quantum states triggered by an unconventional charge density wave (CDW) order. The three-dimensional (3D) order involves a 2x2x2 phase coherent stacking of 2x2 charge density modulations in the kagome plane at low temperatures, exhibiting a CDW energy gap and evidence for time-reversal symmetry breaking. Here we report the discovery of emergent superconductivity and primary pair density wave (PDW) at the antiphase boundaries and stacking faults of bulk CDW order. We find that the π-phase shift dislocations can naturally appear on the surface as the Cs atoms form 2x2 superstructures that are out of phase with the bulk CDW. An incipient narrow band of surface states inside bulk CDW gap emerge close to the Fermi level where a particle-hole symmetric energy gap develops. We demonstrate that the energy gap originates from a novel quasi-2D kagome superconducting state (Tc ~ 5.4 K) intertwined with bulk CDW order, exhibiting an unprecedented vortex core spectrum and spatial modulations of the superconducting gap consistent with a 4x4 PDW. Intriguingly, the 2D kagome superconductivity is shown to be tunable on and off by atomically manipulating the Cs atoms on the surface. Our findings provide fresh new insights for understanding the interplay between the unconventional CDW and superconductivity in kagome metals and a pathway for atomic manipulation and topological defects engineering of quantum many-body states in correlated materials.
title Emergent superconductivity and pair density wave at antiphase boundaries of charge density wave order in kagome metals
topic Superconductivity
url https://arxiv.org/abs/2408.06174