Missing spectral weight in a heavy-fermion system far above Néel temperature

Fuente: arXiv
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Autori principali: Li, Jingwen, Priyadarshi, Debankit, Yang, Chia-Jung, Pohl, Ulli, Stockert, Oliver, von Löhneysen, Hilbert, Pal, Shovon, Fiebig, Manfred, Kroha, Johann
Natura: Preprint
Pubblicazione: 2024
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author Li, Jingwen
Priyadarshi, Debankit
Yang, Chia-Jung
Pohl, Ulli
Stockert, Oliver
von Löhneysen, Hilbert
Pal, Shovon
Fiebig, Manfred
Kroha, Johann
author_facet Li, Jingwen
Priyadarshi, Debankit
Yang, Chia-Jung
Pohl, Ulli
Stockert, Oliver
von Löhneysen, Hilbert
Pal, Shovon
Fiebig, Manfred
Kroha, Johann
contents The competition between the Kondo spin-screening effect and the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction in heavy-fermion systems drives the quantum phase transition between the magnetically ordered and the heavy-Fermi-liquid ground states. Despite intensive investigations of heavy quasiparticles on the Kondo-screened side of the quantum phase transition and of their breakdown at the quantum critical point, the magnetically ordering side has not systematically been studied. Using terahertz time-domain spectroscopy, we report a suppression of the Kondo quasiparticle weight in CeCu$_{6-x}$Au$_x$ samples on the antiferromagnetic side of the quantum phase transition at temperatures as much as two orders of magnitude above the Néel temperature $T_\text{N}$. With our systematic investigations into the high-temperature, paramagnetic region on the antiferromagnetic side of the phase diagram of CeCu$_{6-x}$Au$_x$, i.e., with $x =$ 0.2, 0.3, and 0.5, we show that the suppression results from a quantum frustration effect induced by the temperature-independent RKKY interaction. Hence, our results emphasize that besides critical fluctuations, the RKKY interaction may play an important role in the quantum-critical scenario.
format Preprint
id arxiv_https___arxiv_org_abs_2408_07345
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Missing spectral weight in a heavy-fermion system far above Néel temperature
Li, Jingwen
Priyadarshi, Debankit
Yang, Chia-Jung
Pohl, Ulli
Stockert, Oliver
von Löhneysen, Hilbert
Pal, Shovon
Fiebig, Manfred
Kroha, Johann
Strongly Correlated Electrons
The competition between the Kondo spin-screening effect and the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction in heavy-fermion systems drives the quantum phase transition between the magnetically ordered and the heavy-Fermi-liquid ground states. Despite intensive investigations of heavy quasiparticles on the Kondo-screened side of the quantum phase transition and of their breakdown at the quantum critical point, the magnetically ordering side has not systematically been studied. Using terahertz time-domain spectroscopy, we report a suppression of the Kondo quasiparticle weight in CeCu$_{6-x}$Au$_x$ samples on the antiferromagnetic side of the quantum phase transition at temperatures as much as two orders of magnitude above the Néel temperature $T_\text{N}$. With our systematic investigations into the high-temperature, paramagnetic region on the antiferromagnetic side of the phase diagram of CeCu$_{6-x}$Au$_x$, i.e., with $x =$ 0.2, 0.3, and 0.5, we show that the suppression results from a quantum frustration effect induced by the temperature-independent RKKY interaction. Hence, our results emphasize that besides critical fluctuations, the RKKY interaction may play an important role in the quantum-critical scenario.
title Missing spectral weight in a heavy-fermion system far above Néel temperature
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2408.07345