Altermagnetism in the layered intercalated transition metal dichalcogenide CoNb$_4$Se$_8$

Fuente: arXiv
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Autori principali: Regmi, Resham Babu, Bhandari, Hari, Thapa, Bishal, Hao, Yiqing, Sharma, Nileema, McKenzie, James, Chen, Xinglong, Nayak, Abhijeet, Gazzah, Mohamed El, Márkus, Bence Gábor, Forró, László, Liu, Xiaolong, Cao, Huibo, Mitchell, J. F., Mazin, I. I., Ghimire, Nirmal J.
Natura: Preprint
Pubblicazione: 2024
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author Regmi, Resham Babu
Bhandari, Hari
Thapa, Bishal
Hao, Yiqing
Sharma, Nileema
McKenzie, James
Chen, Xinglong
Nayak, Abhijeet
Gazzah, Mohamed El
Márkus, Bence Gábor
Forró, László
Liu, Xiaolong
Cao, Huibo
Mitchell, J. F.
Mazin, I. I.
Ghimire, Nirmal J.
author_facet Regmi, Resham Babu
Bhandari, Hari
Thapa, Bishal
Hao, Yiqing
Sharma, Nileema
McKenzie, James
Chen, Xinglong
Nayak, Abhijeet
Gazzah, Mohamed El
Márkus, Bence Gábor
Forró, László
Liu, Xiaolong
Cao, Huibo
Mitchell, J. F.
Mazin, I. I.
Ghimire, Nirmal J.
contents Altermagnets (AMs) are a new class of magnetic materials that combine the beneficial spintronics properties of ferromagnets and antiferromagnets, garnering significant attention recently. Here, we have identified altermagnetism in a layered intercalated transition metal diselenide, CoNb$_4$Se$_8$, which crystallizes with an ordered sublattice of intercalated Co atoms between NbSe$_2$ layers. Single crystals are synthesized, and the structural characterizations are performed using single crystal diffraction and scanning tunneling microscopy. Magnetic measurements reveal easy-axis antiferromagnetism below 168 K. Density functional theory (DFT) calculations indicate that A-type antiferromagnetic ordering with easy-axis spin direction is the ground state, which is verified through single crystal neutron diffraction experiments. Electronic band structure calculations in this magnetic state display spin-split bands, confirming altermagnetism in this compound. The layered structure of CoNb$_4$Se$_8$ presents a promising platform for testing various predicted properties associated with altermagnetism.
format Preprint
id arxiv_https___arxiv_org_abs_2408_08835
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Altermagnetism in the layered intercalated transition metal dichalcogenide CoNb$_4$Se$_8$
Regmi, Resham Babu
Bhandari, Hari
Thapa, Bishal
Hao, Yiqing
Sharma, Nileema
McKenzie, James
Chen, Xinglong
Nayak, Abhijeet
Gazzah, Mohamed El
Márkus, Bence Gábor
Forró, László
Liu, Xiaolong
Cao, Huibo
Mitchell, J. F.
Mazin, I. I.
Ghimire, Nirmal J.
Strongly Correlated Electrons
Materials Science
Altermagnets (AMs) are a new class of magnetic materials that combine the beneficial spintronics properties of ferromagnets and antiferromagnets, garnering significant attention recently. Here, we have identified altermagnetism in a layered intercalated transition metal diselenide, CoNb$_4$Se$_8$, which crystallizes with an ordered sublattice of intercalated Co atoms between NbSe$_2$ layers. Single crystals are synthesized, and the structural characterizations are performed using single crystal diffraction and scanning tunneling microscopy. Magnetic measurements reveal easy-axis antiferromagnetism below 168 K. Density functional theory (DFT) calculations indicate that A-type antiferromagnetic ordering with easy-axis spin direction is the ground state, which is verified through single crystal neutron diffraction experiments. Electronic band structure calculations in this magnetic state display spin-split bands, confirming altermagnetism in this compound. The layered structure of CoNb$_4$Se$_8$ presents a promising platform for testing various predicted properties associated with altermagnetism.
title Altermagnetism in the layered intercalated transition metal dichalcogenide CoNb$_4$Se$_8$
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2408.08835