Discovery of terahertz-frequency orbitally-coupled magnons in a kagome ferromagnet

Fuente: arXiv
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Autores principales: Che, Mengqian, Chen, Weizhao, Wang, Maoyuan, Bartram, F. Michael, Liu, Liangyang, Dong, Xuebin, Liu, Jinjin, Li, Yidian, Lin, Hao, Wang, Zhiwei, Liu, Enke, Yao, Yugui, Yuan, Zhe, Zhang, Guang-Ming, Yang, Luyi
Formato: Preprint
Publicado: 2024
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author Che, Mengqian
Chen, Weizhao
Wang, Maoyuan
Bartram, F. Michael
Liu, Liangyang
Dong, Xuebin
Liu, Jinjin
Li, Yidian
Lin, Hao
Wang, Zhiwei
Liu, Enke
Yao, Yugui
Yuan, Zhe
Zhang, Guang-Ming
Yang, Luyi
author_facet Che, Mengqian
Chen, Weizhao
Wang, Maoyuan
Bartram, F. Michael
Liu, Liangyang
Dong, Xuebin
Liu, Jinjin
Li, Yidian
Lin, Hao
Wang, Zhiwei
Liu, Enke
Yao, Yugui
Yuan, Zhe
Zhang, Guang-Ming
Yang, Luyi
contents In ferromagnetic materials, magnons - quanta of spin waves - typically resonate in the gigahertz range. Beyond conventional magnons, while theoretical studies have predicted magnons associated with orbital magnetic moments, their direct observation has remained challenging. Here, we present the discovery of two distinct terahertz orbitally-coupled magnon resonances in the topological kagome ferromagnet Co3Sn2S2. Using time-resolved Kerr rotation spectroscopy, we pinpoint two magnon resonances at 0.61 and 0.49 THz at 6 K, surpassing all previously reported magnon resonances in ferromagnets due to strong magnetocrystalline anisotropy. These dual modes originate from the strong coupling of localized spin and orbital magnetic moments. These findings unveil a novel category of magnons stemming from orbital magnetic moments, and position Co3Sn2S2 as a promising candidate for high-speed terahertz spintronic applications
format Preprint
id arxiv_https___arxiv_org_abs_2408_09417
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Discovery of terahertz-frequency orbitally-coupled magnons in a kagome ferromagnet
Che, Mengqian
Chen, Weizhao
Wang, Maoyuan
Bartram, F. Michael
Liu, Liangyang
Dong, Xuebin
Liu, Jinjin
Li, Yidian
Lin, Hao
Wang, Zhiwei
Liu, Enke
Yao, Yugui
Yuan, Zhe
Zhang, Guang-Ming
Yang, Luyi
Strongly Correlated Electrons
In ferromagnetic materials, magnons - quanta of spin waves - typically resonate in the gigahertz range. Beyond conventional magnons, while theoretical studies have predicted magnons associated with orbital magnetic moments, their direct observation has remained challenging. Here, we present the discovery of two distinct terahertz orbitally-coupled magnon resonances in the topological kagome ferromagnet Co3Sn2S2. Using time-resolved Kerr rotation spectroscopy, we pinpoint two magnon resonances at 0.61 and 0.49 THz at 6 K, surpassing all previously reported magnon resonances in ferromagnets due to strong magnetocrystalline anisotropy. These dual modes originate from the strong coupling of localized spin and orbital magnetic moments. These findings unveil a novel category of magnons stemming from orbital magnetic moments, and position Co3Sn2S2 as a promising candidate for high-speed terahertz spintronic applications
title Discovery of terahertz-frequency orbitally-coupled magnons in a kagome ferromagnet
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2408.09417