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Main Authors: Yu, Yalong, Xiong, Bo, Wu, Siqi, Ren, Yekai, Chen, Nuo, Mi, Qingjiao, Zheng, Zhaojie, Lou, Kangping, Wang, Rui, Chu, Tao
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2408.09738
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author Yu, Yalong
Xiong, Bo
Wu, Siqi
Ren, Yekai
Chen, Nuo
Mi, Qingjiao
Zheng, Zhaojie
Lou, Kangping
Wang, Rui
Chu, Tao
author_facet Yu, Yalong
Xiong, Bo
Wu, Siqi
Ren, Yekai
Chen, Nuo
Mi, Qingjiao
Zheng, Zhaojie
Lou, Kangping
Wang, Rui
Chu, Tao
contents LiNbO3 (LN) is renowned for its exceptional ferroelectric properties, particularly its notable linear electro-optical (EO) effect, which is highly advantageous for various applications such as high-speed communication, optical computation, and quantum information processing. Compared to its ferroelectric properties, the magnetism of LN is not attractive enough due to its weak ferromagnetic nature. Theoretical studies suggest that LN may exhibit a novel magnetoelectric coupling via ferroelectrically-induced ferromagnetism. However, this mechanism has not yet been experimentally validated in any materials, presenting significant challenges for research. In this study, we provide the first experimental evidence supporting the mechanism of ferroelectrically-induced ferromagnetism in LN, including observations of the Dzyaloshinskii-Moriya interaction (DMI) and magnetoelectric coupling. Additionally, we have identified various multiferroic skyrmions, within which ferroelectric polarization signals are detectable. These signals can be influenced by the magnetic vortex structures, indicating a magnetoelectric coupling nature. Currently, they are the only multiferroic skyrmions that can keep stable at room temperature. Moreover, these magnetic textures significantly affect the ferroelectric properties, as demonstrated by an enhancement of the linear electro-optic effect of LN by over 200%. Given the novel magnetoelectric coupling mechanism, the potential of multiferroic skyrmions in spintronics and advanced data storage, and the extensive use of LN EO modulators, our research has significant implications for condensed matter physics, multiferroic materials, and optoelectronics.
format Preprint
id arxiv_https___arxiv_org_abs_2408_09738
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Room-Temperature Multiferroic Skyrmions in LiNbO3 with enhancement in electric-optical property
Yu, Yalong
Xiong, Bo
Wu, Siqi
Ren, Yekai
Chen, Nuo
Mi, Qingjiao
Zheng, Zhaojie
Lou, Kangping
Wang, Rui
Chu, Tao
Materials Science
LiNbO3 (LN) is renowned for its exceptional ferroelectric properties, particularly its notable linear electro-optical (EO) effect, which is highly advantageous for various applications such as high-speed communication, optical computation, and quantum information processing. Compared to its ferroelectric properties, the magnetism of LN is not attractive enough due to its weak ferromagnetic nature. Theoretical studies suggest that LN may exhibit a novel magnetoelectric coupling via ferroelectrically-induced ferromagnetism. However, this mechanism has not yet been experimentally validated in any materials, presenting significant challenges for research. In this study, we provide the first experimental evidence supporting the mechanism of ferroelectrically-induced ferromagnetism in LN, including observations of the Dzyaloshinskii-Moriya interaction (DMI) and magnetoelectric coupling. Additionally, we have identified various multiferroic skyrmions, within which ferroelectric polarization signals are detectable. These signals can be influenced by the magnetic vortex structures, indicating a magnetoelectric coupling nature. Currently, they are the only multiferroic skyrmions that can keep stable at room temperature. Moreover, these magnetic textures significantly affect the ferroelectric properties, as demonstrated by an enhancement of the linear electro-optic effect of LN by over 200%. Given the novel magnetoelectric coupling mechanism, the potential of multiferroic skyrmions in spintronics and advanced data storage, and the extensive use of LN EO modulators, our research has significant implications for condensed matter physics, multiferroic materials, and optoelectronics.
title Room-Temperature Multiferroic Skyrmions in LiNbO3 with enhancement in electric-optical property
topic Materials Science
url https://arxiv.org/abs/2408.09738