How to use the dispersion in the $χ^{(3)}$ tensor for broadband generation of polarization-entangled photons

Fuente: arXiv
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Autori principali: Vento, Valeria, Ciccarello, Francesco, Amirtharaj, Sakthi Pryia, Galland, Christophe
Natura: Preprint
Pubblicazione: 2024
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author Vento, Valeria
Ciccarello, Francesco
Amirtharaj, Sakthi Pryia
Galland, Christophe
author_facet Vento, Valeria
Ciccarello, Francesco
Amirtharaj, Sakthi Pryia
Galland, Christophe
contents Polarization-entangled photon pairs are a widely used resource in quantum optics and technologies, and are often produced using a nonlinear process. Most sources based on spontaneous parametric downconversion have relatively narrow optical bandwidth because the pump, signal and idler frequencies must satisfy a phase-matching condition. Extending the bandwidth, for example to achieve spectral multiplexing, requires changing some experimental parameters such as temperature, crystal angle, poling period, etc. Here, we demonstrate broadband (tens of THz for each photon) generation of polarization-entangled photon pairs by spontaneous four-wave mixing in a diamond crystal, with a simple colinear geometry requiring no further optical engineering. Our approach leverages the quantum interference between electronic and vibrational contributions to the $χ^{(3)}$ tensor. Entanglement is characterized in a single realization of a Bell test over the entire bandwidth using fiber dispersion spectroscopy and fast single-photon detectors. The results agree with the biphoton wavefunction predicted from the knowledge of the $χ^{(3)}$ and Raman tensors and demonstrate the general applicability of our approach to other crystalline materials.
format Preprint
id arxiv_https___arxiv_org_abs_2408_11477
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle How to use the dispersion in the $χ^{(3)}$ tensor for broadband generation of polarization-entangled photons
Vento, Valeria
Ciccarello, Francesco
Amirtharaj, Sakthi Pryia
Galland, Christophe
Quantum Physics
Materials Science
Optics
Polarization-entangled photon pairs are a widely used resource in quantum optics and technologies, and are often produced using a nonlinear process. Most sources based on spontaneous parametric downconversion have relatively narrow optical bandwidth because the pump, signal and idler frequencies must satisfy a phase-matching condition. Extending the bandwidth, for example to achieve spectral multiplexing, requires changing some experimental parameters such as temperature, crystal angle, poling period, etc. Here, we demonstrate broadband (tens of THz for each photon) generation of polarization-entangled photon pairs by spontaneous four-wave mixing in a diamond crystal, with a simple colinear geometry requiring no further optical engineering. Our approach leverages the quantum interference between electronic and vibrational contributions to the $χ^{(3)}$ tensor. Entanglement is characterized in a single realization of a Bell test over the entire bandwidth using fiber dispersion spectroscopy and fast single-photon detectors. The results agree with the biphoton wavefunction predicted from the knowledge of the $χ^{(3)}$ and Raman tensors and demonstrate the general applicability of our approach to other crystalline materials.
title How to use the dispersion in the $χ^{(3)}$ tensor for broadband generation of polarization-entangled photons
topic Quantum Physics
Materials Science
Optics
url https://arxiv.org/abs/2408.11477