Tunneling photo-thermoelectric effect in monolayer graphene/bilayer hexagonal boron nitride/bilayer graphene asymmetric van der Waals tunnel junctions

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Hauptverfasser: Park, Sabin, Moriya, Rai, Zhang, Yijin, Watanabe, Kenji, Taniguchi, Takashi, Machida, Tomoki
Format: Preprint
Veröffentlicht: 2024
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author Park, Sabin
Moriya, Rai
Zhang, Yijin
Watanabe, Kenji
Taniguchi, Takashi
Machida, Tomoki
author_facet Park, Sabin
Moriya, Rai
Zhang, Yijin
Watanabe, Kenji
Taniguchi, Takashi
Machida, Tomoki
contents Graphene is known to exhibit a pronounced photo-thermoelectric effect (PTE) in its in-plane carrier transport and attracting attention toward various optoelectronic applications. In this study, we demonstrate an out-of-plane PTE by utilizing electron tunneling across a barrier, namely, the tunneling photo-thermoelectric effect (TPTE). This was achieved in a monolayer graphene (MLG)/bilayer hexagonal boron nitride (h-BN)/bilayer graphene (BLG) asymmetric tunnel junction. MLG and BLG exhibit different cyclotron resonance (CR) optical absorption energies when their energies are Landau quantized under an out-of-plane magnetic field. We tuned the magnetic field under mid-infrared (MIR) irradiation to bring MLG into CR conditions, whereas BLG was not in CR. The CR absorption in the MLG generates an electron temperature difference between the MLG and BLG, and induces an out-of-plane TPTE voltage across the h-BN tunnel barrier. The TPTE exhibited a unique dependence on the Fermi energy of the MLG, which differed from that of the in-plane PTE of the MLG. The TPTE signal was large when the Fermi energy of the MLG was tuned near the phase transition between the quantum Hall state (QHS) and non-QHS, that is, the transition between carrier localization and delocalization. The TPTE provides another degree of freedom for probing the electronic and optoelectronic properties of two-dimensional material heterostructures.
format Preprint
id arxiv_https___arxiv_org_abs_2408_12501
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Tunneling photo-thermoelectric effect in monolayer graphene/bilayer hexagonal boron nitride/bilayer graphene asymmetric van der Waals tunnel junctions
Park, Sabin
Moriya, Rai
Zhang, Yijin
Watanabe, Kenji
Taniguchi, Takashi
Machida, Tomoki
Mesoscale and Nanoscale Physics
Graphene is known to exhibit a pronounced photo-thermoelectric effect (PTE) in its in-plane carrier transport and attracting attention toward various optoelectronic applications. In this study, we demonstrate an out-of-plane PTE by utilizing electron tunneling across a barrier, namely, the tunneling photo-thermoelectric effect (TPTE). This was achieved in a monolayer graphene (MLG)/bilayer hexagonal boron nitride (h-BN)/bilayer graphene (BLG) asymmetric tunnel junction. MLG and BLG exhibit different cyclotron resonance (CR) optical absorption energies when their energies are Landau quantized under an out-of-plane magnetic field. We tuned the magnetic field under mid-infrared (MIR) irradiation to bring MLG into CR conditions, whereas BLG was not in CR. The CR absorption in the MLG generates an electron temperature difference between the MLG and BLG, and induces an out-of-plane TPTE voltage across the h-BN tunnel barrier. The TPTE exhibited a unique dependence on the Fermi energy of the MLG, which differed from that of the in-plane PTE of the MLG. The TPTE signal was large when the Fermi energy of the MLG was tuned near the phase transition between the quantum Hall state (QHS) and non-QHS, that is, the transition between carrier localization and delocalization. The TPTE provides another degree of freedom for probing the electronic and optoelectronic properties of two-dimensional material heterostructures.
title Tunneling photo-thermoelectric effect in monolayer graphene/bilayer hexagonal boron nitride/bilayer graphene asymmetric van der Waals tunnel junctions
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2408.12501