Unidirectional chiral scattering from single enantiomeric plasmonic nanoparticles

Fuente: arXiv
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Autores principales: Xie, Yuanyang, Krasavin, Alexey V., Roth, Diane J., Zayats, Anatoly V.
Formato: Preprint
Publicado: 2024
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author Xie, Yuanyang
Krasavin, Alexey V.
Roth, Diane J.
Zayats, Anatoly V.
author_facet Xie, Yuanyang
Krasavin, Alexey V.
Roth, Diane J.
Zayats, Anatoly V.
contents Controlling scattering and routing of chiral light at the nanoscale is important for optical information processing and imaging, quantum technologies as well as optical manipulation. Here, we introduce a concept of rotating chiral dipoles in order to achieve unidirectional chiral scattering. Implementing this concept by engineering multipole excitations in plasmonic helicoidal nanoparticles, we experimentally demonstrate enantio-sensitive and highly-directional forward scattering of circularly polarised light. The intensity of this highly-directional scattering is defined by the mutual relation between the handedness of the incident light and the chirality of the structure. The concept of rotating chiral dipoles opens up numerous possibilities for engineering of scattering from chiral nanostructures and optical nano-antennas for the design and application of chiral light-matter interaction.
format Preprint
id arxiv_https___arxiv_org_abs_2408_14376
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Unidirectional chiral scattering from single enantiomeric plasmonic nanoparticles
Xie, Yuanyang
Krasavin, Alexey V.
Roth, Diane J.
Zayats, Anatoly V.
Optics
Controlling scattering and routing of chiral light at the nanoscale is important for optical information processing and imaging, quantum technologies as well as optical manipulation. Here, we introduce a concept of rotating chiral dipoles in order to achieve unidirectional chiral scattering. Implementing this concept by engineering multipole excitations in plasmonic helicoidal nanoparticles, we experimentally demonstrate enantio-sensitive and highly-directional forward scattering of circularly polarised light. The intensity of this highly-directional scattering is defined by the mutual relation between the handedness of the incident light and the chirality of the structure. The concept of rotating chiral dipoles opens up numerous possibilities for engineering of scattering from chiral nanostructures and optical nano-antennas for the design and application of chiral light-matter interaction.
title Unidirectional chiral scattering from single enantiomeric plasmonic nanoparticles
topic Optics
url https://arxiv.org/abs/2408.14376