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Ionization potential of radium monofluoride

Fuente: arXiv
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Autori principali: Wilkins, S. G., Perrett, H. A., Udrescu, S. M., Kyuberis, A. A., Pašteka, L. F., Au, M., Belošević, I., Berger, R., Binnersley, C. L., Bissell, M. L., Borschevsky, A., Breier, A. A., Brinson, A. J., Chrysalidis, K., Cocolios, T. E., Cooper, B. S., de Groote, R. P., Dorne, A., Eliav, E., Field, R. W., Flanagan, K. T., Franchoo, S., Ruiz, R. F. Garcia, Gaul, K., Geldhof, S., Giesen, T. F., Gustafsson, F. P., Hanstorp, D., Heinke, R., Koszorús, Á., Kujanpää, S., Lalanne, L., Neyens, G., Nichols, M., Reilly, J. R., Ricketts, C. M., Rothe, S., Sunaga, A., Borne, B. van den, Vernon, A. R., Wang, Q., Wessolek, J., Wienholtz, F., Yang, X. F., Zhou, Y., Zülch, C.
Natura: Preprint
Pubblicazione: 2024
Soggetti:
Atomic Physics
Nuclear Experiment
Chemical Physics
Computational Physics
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_version_ 1866911374166196224
author Wilkins, S. G.
Perrett, H. A.
Udrescu, S. M.
Kyuberis, A. A.
Pašteka, L. F.
Au, M.
Belošević, I.
Berger, R.
Binnersley, C. L.
Bissell, M. L.
Borschevsky, A.
Breier, A. A.
Brinson, A. J.
Chrysalidis, K.
Cocolios, T. E.
Cooper, B. S.
de Groote, R. P.
Dorne, A.
Eliav, E.
Field, R. W.
Flanagan, K. T.
Franchoo, S.
Ruiz, R. F. Garcia
Gaul, K.
Geldhof, S.
Giesen, T. F.
Gustafsson, F. P.
Hanstorp, D.
Heinke, R.
Koszorús, Á.
Kujanpää, S.
Lalanne, L.
Neyens, G.
Nichols, M.
Reilly, J. R.
Ricketts, C. M.
Rothe, S.
Sunaga, A.
Borne, B. van den
Vernon, A. R.
Wang, Q.
Wessolek, J.
Wienholtz, F.
Yang, X. F.
Zhou, Y.
Zülch, C.
author_facet Wilkins, S. G.
Perrett, H. A.
Udrescu, S. M.
Kyuberis, A. A.
Pašteka, L. F.
Au, M.
Belošević, I.
Berger, R.
Binnersley, C. L.
Bissell, M. L.
Borschevsky, A.
Breier, A. A.
Brinson, A. J.
Chrysalidis, K.
Cocolios, T. E.
Cooper, B. S.
de Groote, R. P.
Dorne, A.
Eliav, E.
Field, R. W.
Flanagan, K. T.
Franchoo, S.
Ruiz, R. F. Garcia
Gaul, K.
Geldhof, S.
Giesen, T. F.
Gustafsson, F. P.
Hanstorp, D.
Heinke, R.
Koszorús, Á.
Kujanpää, S.
Lalanne, L.
Neyens, G.
Nichols, M.
Reilly, J. R.
Ricketts, C. M.
Rothe, S.
Sunaga, A.
Borne, B. van den
Vernon, A. R.
Wang, Q.
Wessolek, J.
Wienholtz, F.
Yang, X. F.
Zhou, Y.
Zülch, C.
contents The ionization potential (IP) of radium monofluoride (RaF) was measured to be 4.969(2)[10] eV, revealing a relativistic enhancement in the series of alkaline earth monofluorides. The results are in agreement with a relativistic coupled-cluster prediction of 4.969[7] eV, incorporating up to quantum electrodynamics corrections. Using the same computational methodology, an improved calculation for the dissociation energy ($D_{0}$) of 5.54[5] eV is presented. This confirms that radium monofluoride joins the small group of diatomic molecules for which $D_{0}>\mathrm{IP}$, paving the way for precision control and interrogation of its Rydberg states.
format Preprint
id arxiv_https___arxiv_org_abs_2408_14673
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Ionization potential of radium monofluoride
Wilkins, S. G.
Perrett, H. A.
Udrescu, S. M.
Kyuberis, A. A.
Pašteka, L. F.
Au, M.
Belošević, I.
Berger, R.
Binnersley, C. L.
Bissell, M. L.
Borschevsky, A.
Breier, A. A.
Brinson, A. J.
Chrysalidis, K.
Cocolios, T. E.
Cooper, B. S.
de Groote, R. P.
Dorne, A.
Eliav, E.
Field, R. W.
Flanagan, K. T.
Franchoo, S.
Ruiz, R. F. Garcia
Gaul, K.
Geldhof, S.
Giesen, T. F.
Gustafsson, F. P.
Hanstorp, D.
Heinke, R.
Koszorús, Á.
Kujanpää, S.
Lalanne, L.
Neyens, G.
Nichols, M.
Reilly, J. R.
Ricketts, C. M.
Rothe, S.
Sunaga, A.
Borne, B. van den
Vernon, A. R.
Wang, Q.
Wessolek, J.
Wienholtz, F.
Yang, X. F.
Zhou, Y.
Zülch, C.
Atomic Physics
Nuclear Experiment
Chemical Physics
Computational Physics
The ionization potential (IP) of radium monofluoride (RaF) was measured to be 4.969(2)[10] eV, revealing a relativistic enhancement in the series of alkaline earth monofluorides. The results are in agreement with a relativistic coupled-cluster prediction of 4.969[7] eV, incorporating up to quantum electrodynamics corrections. Using the same computational methodology, an improved calculation for the dissociation energy ($D_{0}$) of 5.54[5] eV is presented. This confirms that radium monofluoride joins the small group of diatomic molecules for which $D_{0}>\mathrm{IP}$, paving the way for precision control and interrogation of its Rydberg states.
title Ionization potential of radium monofluoride
topic Atomic Physics
Nuclear Experiment
Chemical Physics
Computational Physics
url https://arxiv.org/abs/2408.14673

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