Signatures of Chiral Superconductivity in Rhombohedral Graphene

Fuente: arXiv
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Main Authors: Han, Tonghang, Lu, Zhengguang, Hadjri, Zach, Shi, Lihan, Wu, Zhenghan, Xu, Wei, Yao, Yuxuan, Cotten, Armel A., Sedeh, Omid Sharifi, Weldeyesus, Henok, Yang, Jixiang, Seo, Junseok, Ye, Shenyong, Zhou, Muyang, Liu, Haoyang, Shi, Gang, Hua, Zhenqi, Watanabe, Kenji, Taniguchi, Takashi, Xiong, Peng, Zumbühl, Dominik M., Fu, Liang, Ju, Long
Format: Preprint
Published: 2024
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author Han, Tonghang
Lu, Zhengguang
Hadjri, Zach
Shi, Lihan
Wu, Zhenghan
Xu, Wei
Yao, Yuxuan
Cotten, Armel A.
Sedeh, Omid Sharifi
Weldeyesus, Henok
Yang, Jixiang
Seo, Junseok
Ye, Shenyong
Zhou, Muyang
Liu, Haoyang
Shi, Gang
Hua, Zhenqi
Watanabe, Kenji
Taniguchi, Takashi
Xiong, Peng
Zumbühl, Dominik M.
Fu, Liang
Ju, Long
author_facet Han, Tonghang
Lu, Zhengguang
Hadjri, Zach
Shi, Lihan
Wu, Zhenghan
Xu, Wei
Yao, Yuxuan
Cotten, Armel A.
Sedeh, Omid Sharifi
Weldeyesus, Henok
Yang, Jixiang
Seo, Junseok
Ye, Shenyong
Zhou, Muyang
Liu, Haoyang
Shi, Gang
Hua, Zhenqi
Watanabe, Kenji
Taniguchi, Takashi
Xiong, Peng
Zumbühl, Dominik M.
Fu, Liang
Ju, Long
contents Chiral superconductors are unconventional superconducting states that break time reversal symmetry spontaneously and typically feature Cooper pairing at non-zero angular momentum. Such states may host Majorana fermions and provide an important platform for topological physics research and fault-tolerant quantum computing. Despite intensive search and prolonged studies of several candidate systems, chiral superconductivity has remained elusive so far. Here we report the discovery of robust unconventional superconductivity in rhombohedral tetra- and penta-layer graphene in the absence of moiré superlattice effects. We observed two superconducting states in the gate-induced flat conduction bands with Tc up to 300 mK and charge density ne as low as 2.4*1011 cm-2 in three tetralayer and two pentalayer devices. Spontaneous time-reversal-symmetry-breaking (TRSB) due to electron's orbital motion is found, and several observations indicate the chiral nature of these superconducting states, including: 1. In the superconducting state, Rxx shows magnetic hysteresis in varying out-of-plane magnetic field B, which is absent from all other superconductors; 2. the superconducting states are immune to in-plane magnetic field and are developed within a spin- and valley-polarized quarter-metal phase; 3. the normal states show anomalous Hall signals at zero magnetic field and magnetic hysteresis. We also observed a critical B of up to 1.4 Tesla, higher than any graphene superconductivity reported so far and indicates a strong-coupling superconductivity close to the BCS-BEC crossover. Our observations establish a pure carbon material for the study of topological superconductivity, and pave the way to explore Majorana modes and topological quantum computing.
format Preprint
id arxiv_https___arxiv_org_abs_2408_15233
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Signatures of Chiral Superconductivity in Rhombohedral Graphene
Han, Tonghang
Lu, Zhengguang
Hadjri, Zach
Shi, Lihan
Wu, Zhenghan
Xu, Wei
Yao, Yuxuan
Cotten, Armel A.
Sedeh, Omid Sharifi
Weldeyesus, Henok
Yang, Jixiang
Seo, Junseok
Ye, Shenyong
Zhou, Muyang
Liu, Haoyang
Shi, Gang
Hua, Zhenqi
Watanabe, Kenji
Taniguchi, Takashi
Xiong, Peng
Zumbühl, Dominik M.
Fu, Liang
Ju, Long
Mesoscale and Nanoscale Physics
Chiral superconductors are unconventional superconducting states that break time reversal symmetry spontaneously and typically feature Cooper pairing at non-zero angular momentum. Such states may host Majorana fermions and provide an important platform for topological physics research and fault-tolerant quantum computing. Despite intensive search and prolonged studies of several candidate systems, chiral superconductivity has remained elusive so far. Here we report the discovery of robust unconventional superconductivity in rhombohedral tetra- and penta-layer graphene in the absence of moiré superlattice effects. We observed two superconducting states in the gate-induced flat conduction bands with Tc up to 300 mK and charge density ne as low as 2.4*1011 cm-2 in three tetralayer and two pentalayer devices. Spontaneous time-reversal-symmetry-breaking (TRSB) due to electron's orbital motion is found, and several observations indicate the chiral nature of these superconducting states, including: 1. In the superconducting state, Rxx shows magnetic hysteresis in varying out-of-plane magnetic field B, which is absent from all other superconductors; 2. the superconducting states are immune to in-plane magnetic field and are developed within a spin- and valley-polarized quarter-metal phase; 3. the normal states show anomalous Hall signals at zero magnetic field and magnetic hysteresis. We also observed a critical B of up to 1.4 Tesla, higher than any graphene superconductivity reported so far and indicates a strong-coupling superconductivity close to the BCS-BEC crossover. Our observations establish a pure carbon material for the study of topological superconductivity, and pave the way to explore Majorana modes and topological quantum computing.
title Signatures of Chiral Superconductivity in Rhombohedral Graphene
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2408.15233