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Main Authors: Wu, Di, Bai, C. L., Sagawa, H., Zhang, H. Q.
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2408.16523
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author Wu, Di
Bai, C. L.
Sagawa, H.
Zhang, H. Q.
author_facet Wu, Di
Bai, C. L.
Sagawa, H.
Zhang, H. Q.
contents We implement the Multi-Reference Unitary Coupled Cluster Singles and Doubles (MR-UCCSD) model with a quantum circuit that conserves the particle number to study the ground state energies of LiH, BeH$_2$, and H$_6$. This approach simplifies the MR-UCCSD computation by integrating quantum computing techniques, and reduces its complexity. As a profit of the better MR states, our MR-UCCSD approach satisfies systematically the predefined errors below 10$^{-5}$ Hartree,which is the highest precision of single reference UCCSD approach, along the whole bond length with only hundreds of CNOT gates, and meets satisfactory the requirements of both computational precision and quantum resource reduction.
format Preprint
id arxiv_https___arxiv_org_abs_2408_16523
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Multi-Reference UCCSD Variational Quantum Algorithm for Molecular Ground State Energies
Wu, Di
Bai, C. L.
Sagawa, H.
Zhang, H. Q.
Quantum Physics
We implement the Multi-Reference Unitary Coupled Cluster Singles and Doubles (MR-UCCSD) model with a quantum circuit that conserves the particle number to study the ground state energies of LiH, BeH$_2$, and H$_6$. This approach simplifies the MR-UCCSD computation by integrating quantum computing techniques, and reduces its complexity. As a profit of the better MR states, our MR-UCCSD approach satisfies systematically the predefined errors below 10$^{-5}$ Hartree,which is the highest precision of single reference UCCSD approach, along the whole bond length with only hundreds of CNOT gates, and meets satisfactory the requirements of both computational precision and quantum resource reduction.
title Multi-Reference UCCSD Variational Quantum Algorithm for Molecular Ground State Energies
topic Quantum Physics
url https://arxiv.org/abs/2408.16523