Structural Evolution from Hyper-Honeycomb to Honeycomb Networks and Superconductivity in LaPt$_x$Si$_{2-x}$

Fuente: arXiv
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Auteurs principaux: Ramakrishnan, Sitaram, Yamakawa, Tatsuya, Oishi, Ryohei, Yamane, Soichiro, Ikeda, Atsutoshi, Kado, Masaki, Shimura, Yasuyuki, Takabatake, Toshiro, Onimaru, Takahiro, Shibata, Yasuhiro, Thamizhavel, Arumugam, Ramakrishnan, Srinivasan, Yonezawa, Shingo, Nohara, Minoru
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Publié: 2024
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author Ramakrishnan, Sitaram
Yamakawa, Tatsuya
Oishi, Ryohei
Yamane, Soichiro
Ikeda, Atsutoshi
Kado, Masaki
Shimura, Yasuyuki
Takabatake, Toshiro
Onimaru, Takahiro
Shibata, Yasuhiro
Thamizhavel, Arumugam
Ramakrishnan, Srinivasan
Yonezawa, Shingo
Nohara, Minoru
author_facet Ramakrishnan, Sitaram
Yamakawa, Tatsuya
Oishi, Ryohei
Yamane, Soichiro
Ikeda, Atsutoshi
Kado, Masaki
Shimura, Yasuyuki
Takabatake, Toshiro
Onimaru, Takahiro
Shibata, Yasuhiro
Thamizhavel, Arumugam
Ramakrishnan, Srinivasan
Yonezawa, Shingo
Nohara, Minoru
contents We report the crystal structures and superconductivity (SC) of LaPt$_{x}$Si$_{2-x}$ ($0.5 \leq x \leq 1.0$) that are solid solutions of LaSi$_{2}$ and LaPtSi with centrosymmetric tetragonal ($I4_{1}/amd$, $D_{4h}^{19}$, \#141) and non-centrosymmetric tetragonal ($I4_{1}md$, $C_{4v}^{11}$, \#109) structures, respectively. It was found that at $0.86 \leq x \leq 1.00$, the non-centrosymmetric tetragonal symmetry is preserved, while partial disorder appears in alternating Pt and Si of the hyper-honeycomb network. The superconducting transition temperature $T_{\rm c}$ was drastically reduced from 3.9 K to 1.5 K as $x$ varies from 1.0 to 0.86. Additionally, a hexagonal phase with an AlB$_{2}$-type structure ($P6/mmm$, $D_{6h}^{1}$, \#191) has been discovered at $0.50 \leq x \leq 0.71$ with a honeycomb network of statistically distributed Pt and Si atoms. The hexagonal phase exhibited SC at $T_{\rm c} = 0.38$ K. This system provides an opportunity to investigate the relationship between topological electronic states, SC, and disorders
format Preprint
id arxiv_https___arxiv_org_abs_2408_17033
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Structural Evolution from Hyper-Honeycomb to Honeycomb Networks and Superconductivity in LaPt$_x$Si$_{2-x}$
Ramakrishnan, Sitaram
Yamakawa, Tatsuya
Oishi, Ryohei
Yamane, Soichiro
Ikeda, Atsutoshi
Kado, Masaki
Shimura, Yasuyuki
Takabatake, Toshiro
Onimaru, Takahiro
Shibata, Yasuhiro
Thamizhavel, Arumugam
Ramakrishnan, Srinivasan
Yonezawa, Shingo
Nohara, Minoru
Superconductivity
Strongly Correlated Electrons
We report the crystal structures and superconductivity (SC) of LaPt$_{x}$Si$_{2-x}$ ($0.5 \leq x \leq 1.0$) that are solid solutions of LaSi$_{2}$ and LaPtSi with centrosymmetric tetragonal ($I4_{1}/amd$, $D_{4h}^{19}$, \#141) and non-centrosymmetric tetragonal ($I4_{1}md$, $C_{4v}^{11}$, \#109) structures, respectively. It was found that at $0.86 \leq x \leq 1.00$, the non-centrosymmetric tetragonal symmetry is preserved, while partial disorder appears in alternating Pt and Si of the hyper-honeycomb network. The superconducting transition temperature $T_{\rm c}$ was drastically reduced from 3.9 K to 1.5 K as $x$ varies from 1.0 to 0.86. Additionally, a hexagonal phase with an AlB$_{2}$-type structure ($P6/mmm$, $D_{6h}^{1}$, \#191) has been discovered at $0.50 \leq x \leq 0.71$ with a honeycomb network of statistically distributed Pt and Si atoms. The hexagonal phase exhibited SC at $T_{\rm c} = 0.38$ K. This system provides an opportunity to investigate the relationship between topological electronic states, SC, and disorders
title Structural Evolution from Hyper-Honeycomb to Honeycomb Networks and Superconductivity in LaPt$_x$Si$_{2-x}$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2408.17033