Electron volt energy resolution with ptychography using a broadband continuum spectrum

Fuente: arXiv
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Autori principali: Cipiccia, Silvia, Stolp, Wiebe, Fardin, Luca, Ziesche, Ralf, Manke, Ingo, Boone, Matthieu, Armstrong, Chris, Olivo, Alessandro, Batey, Darren
Natura: Preprint
Pubblicazione: 2024
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author Cipiccia, Silvia
Stolp, Wiebe
Fardin, Luca
Ziesche, Ralf
Manke, Ingo
Boone, Matthieu
Armstrong, Chris
Olivo, Alessandro
Batey, Darren
author_facet Cipiccia, Silvia
Stolp, Wiebe
Fardin, Luca
Ziesche, Ralf
Manke, Ingo
Boone, Matthieu
Armstrong, Chris
Olivo, Alessandro
Batey, Darren
contents Ptychography is a scanning coherent diffraction imaging technique successfully applied in the electron, visible and x-ray regimes. One of the distinct features of ptychography with respect to other coherent diffraction techniques is its capability of dealing with partial spatial and temporal coherence via the reconstruction algorithm. Here we focus on the temporal and clarify theoretically and with simulations the constraints which affect the energy resolution limits of the ptychographic algorithms. Based on this, we design and perform simulations for a broadband ptychography in the hard x-ray regime, which enables an energy resolution down to 1 eV. We benchmark the simulations against experimental ptychographic data from a nickel test sample, by extracting the x-ray absorption near edge spectrum with energy resolution of 5 eV using a continuum spectrum of 20 eV bandwidth. We review the results, discuss the limitations, and provide guidelines for future broadband ptychography experiments, its prospective applications and potential impact on achieving diffraction limited resolutions.
format Preprint
id arxiv_https___arxiv_org_abs_2409_00703
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Electron volt energy resolution with ptychography using a broadband continuum spectrum
Cipiccia, Silvia
Stolp, Wiebe
Fardin, Luca
Ziesche, Ralf
Manke, Ingo
Boone, Matthieu
Armstrong, Chris
Olivo, Alessandro
Batey, Darren
Applied Physics
Computational Physics
Ptychography is a scanning coherent diffraction imaging technique successfully applied in the electron, visible and x-ray regimes. One of the distinct features of ptychography with respect to other coherent diffraction techniques is its capability of dealing with partial spatial and temporal coherence via the reconstruction algorithm. Here we focus on the temporal and clarify theoretically and with simulations the constraints which affect the energy resolution limits of the ptychographic algorithms. Based on this, we design and perform simulations for a broadband ptychography in the hard x-ray regime, which enables an energy resolution down to 1 eV. We benchmark the simulations against experimental ptychographic data from a nickel test sample, by extracting the x-ray absorption near edge spectrum with energy resolution of 5 eV using a continuum spectrum of 20 eV bandwidth. We review the results, discuss the limitations, and provide guidelines for future broadband ptychography experiments, its prospective applications and potential impact on achieving diffraction limited resolutions.
title Electron volt energy resolution with ptychography using a broadband continuum spectrum
topic Applied Physics
Computational Physics
url https://arxiv.org/abs/2409.00703