Structural Properties and Recrystallization Effects in Ion Beam Modified B20-type FeGe Films

Fuente: arXiv
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Main Authors: Liu, Jiangteng, Schoell, Ryan, Zhang, Xiyue S., Yang, Hongbin, Venuti, M. B., Paik, Hanjong, Muller, David A., Lu, Tzu-Ming, Hattar, Khalid, Eley, Serena
Format: Preprint
Published: 2024
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author Liu, Jiangteng
Schoell, Ryan
Zhang, Xiyue S.
Yang, Hongbin
Venuti, M. B.
Paik, Hanjong
Muller, David A.
Lu, Tzu-Ming
Hattar, Khalid
Eley, Serena
author_facet Liu, Jiangteng
Schoell, Ryan
Zhang, Xiyue S.
Yang, Hongbin
Venuti, M. B.
Paik, Hanjong
Muller, David A.
Lu, Tzu-Ming
Hattar, Khalid
Eley, Serena
contents Disordered iron germanium (FeGe) has recently garnered interest as a testbed for a variety of magnetic phenomena as well as for use in magnetic memory and logic applications. This is partially owing to its ability to host skyrmions and antiskyrmions -- nanoscale whirlpools of magnetic moments that could serve as information carriers in spintronic devices. In particular, a tunable skyrmion-antiskyrmion system may be created through precise control of the defect landscape in B20-phase FeGe, motivating developing methods to systematically tune disorder in this material and understand the ensuing structural properties. To this end, we investigate a route for modifying magnetic properties in FeGe. Specifically, we irradiate epitaxial B20-phase FeGe films with 2.8 MeV Au$^{4+}$ ions, which creates a dispersion of amorphized regions that may preferentially host antiskyrmions at densities controlled by the irradiation fluence. To further tune the disorder landscape, we conduct a systematic electron diffraction study with in-situ annealing, demonstrating the ability to recrystallize controllable fractions of the material at temperatures ranging from approximately 150$^{\circ}$ C to 250$^{\circ}$C. Finally, we describe the crystallization kinetics using the Johnson-Mehl-Avrami-Kolmogorov model, finding that the growth of crystalline grains is consistent with diffusion-controlled one-to-two dimensional growth with a decreasing nucleation rate.
format Preprint
id arxiv_https___arxiv_org_abs_2409_02325
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Structural Properties and Recrystallization Effects in Ion Beam Modified B20-type FeGe Films
Liu, Jiangteng
Schoell, Ryan
Zhang, Xiyue S.
Yang, Hongbin
Venuti, M. B.
Paik, Hanjong
Muller, David A.
Lu, Tzu-Ming
Hattar, Khalid
Eley, Serena
Materials Science
Mesoscale and Nanoscale Physics
Disordered iron germanium (FeGe) has recently garnered interest as a testbed for a variety of magnetic phenomena as well as for use in magnetic memory and logic applications. This is partially owing to its ability to host skyrmions and antiskyrmions -- nanoscale whirlpools of magnetic moments that could serve as information carriers in spintronic devices. In particular, a tunable skyrmion-antiskyrmion system may be created through precise control of the defect landscape in B20-phase FeGe, motivating developing methods to systematically tune disorder in this material and understand the ensuing structural properties. To this end, we investigate a route for modifying magnetic properties in FeGe. Specifically, we irradiate epitaxial B20-phase FeGe films with 2.8 MeV Au$^{4+}$ ions, which creates a dispersion of amorphized regions that may preferentially host antiskyrmions at densities controlled by the irradiation fluence. To further tune the disorder landscape, we conduct a systematic electron diffraction study with in-situ annealing, demonstrating the ability to recrystallize controllable fractions of the material at temperatures ranging from approximately 150$^{\circ}$ C to 250$^{\circ}$C. Finally, we describe the crystallization kinetics using the Johnson-Mehl-Avrami-Kolmogorov model, finding that the growth of crystalline grains is consistent with diffusion-controlled one-to-two dimensional growth with a decreasing nucleation rate.
title Structural Properties and Recrystallization Effects in Ion Beam Modified B20-type FeGe Films
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2409.02325