Electrical control of topological 3Q state in intercalated van der Waals antiferromagnet Cox-TaS2

Fuente: arXiv
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Auteurs principaux: Kim, Junghyun, Zhang, Kai-Xuan, Park, Pyeongjae, Cho, Woonghee, Kim, Hyuncheol, Noh, Han-Jin, Park, Je-Geun
Format: Preprint
Publié: 2024
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author Kim, Junghyun
Zhang, Kai-Xuan
Park, Pyeongjae
Cho, Woonghee
Kim, Hyuncheol
Noh, Han-Jin
Park, Je-Geun
author_facet Kim, Junghyun
Zhang, Kai-Xuan
Park, Pyeongjae
Cho, Woonghee
Kim, Hyuncheol
Noh, Han-Jin
Park, Je-Geun
contents Van der Waals (vdW) magnets have opened a new avenue of opportunities encompassing various interesting phases. Co1/3TaS2-an intercalated metallic vdW antiferromagnet-is one of the latest additions to this growing list of materials due to its unique topologically nontrivial triple-Q (3Q) ground state. This 3Q tetrahedral structure, which critically depends on the Co content, yields the highest-density Skyrmion lattice with scalar spin chirality, resulting in a noticeable anomalous Hall effect. In this work, we demonstrate control of this topological phase via ionic gating. Using four CoxTaS2 devices with different Co compositions, we show that ionic gating can cover the entire 3Q topological phase and reveal the nature of the thermodynamically inaccessible phase space. Another striking finding in our data is the existence of an adiabatic discontinuity in the phase boundary between the 3Q and 1Q phases. Our work constitutes one of the first examples of electrical control of scalar spin chirality using an antiferromagnetic metal.
format Preprint
id arxiv_https___arxiv_org_abs_2409_02710
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Electrical control of topological 3Q state in intercalated van der Waals antiferromagnet Cox-TaS2
Kim, Junghyun
Zhang, Kai-Xuan
Park, Pyeongjae
Cho, Woonghee
Kim, Hyuncheol
Noh, Han-Jin
Park, Je-Geun
Materials Science
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Applied Physics
Quantum Physics
Van der Waals (vdW) magnets have opened a new avenue of opportunities encompassing various interesting phases. Co1/3TaS2-an intercalated metallic vdW antiferromagnet-is one of the latest additions to this growing list of materials due to its unique topologically nontrivial triple-Q (3Q) ground state. This 3Q tetrahedral structure, which critically depends on the Co content, yields the highest-density Skyrmion lattice with scalar spin chirality, resulting in a noticeable anomalous Hall effect. In this work, we demonstrate control of this topological phase via ionic gating. Using four CoxTaS2 devices with different Co compositions, we show that ionic gating can cover the entire 3Q topological phase and reveal the nature of the thermodynamically inaccessible phase space. Another striking finding in our data is the existence of an adiabatic discontinuity in the phase boundary between the 3Q and 1Q phases. Our work constitutes one of the first examples of electrical control of scalar spin chirality using an antiferromagnetic metal.
title Electrical control of topological 3Q state in intercalated van der Waals antiferromagnet Cox-TaS2
topic Materials Science
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Applied Physics
Quantum Physics
url https://arxiv.org/abs/2409.02710