Origin of the laser-induced picosecond spin current across magnetization compensation in ferrimagnetic GdCo

Fuente: arXiv
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Autores principales: Antonio, Guillermo Nava, Remy, Quentin, Lin, Jun-Xiao, Guen, Yann Le, Hamara, Dominik, Compton-Stewart, Jude, Barker, Joseph, Hauet, Thomas, Hehn, Michel, Mangin, Stéphane, Ciccarelli, Chiara
Formato: Preprint
Publicado: 2024
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author Antonio, Guillermo Nava
Remy, Quentin
Lin, Jun-Xiao
Guen, Yann Le
Hamara, Dominik
Compton-Stewart, Jude
Barker, Joseph
Hauet, Thomas
Hehn, Michel
Mangin, Stéphane
Ciccarelli, Chiara
author_facet Antonio, Guillermo Nava
Remy, Quentin
Lin, Jun-Xiao
Guen, Yann Le
Hamara, Dominik
Compton-Stewart, Jude
Barker, Joseph
Hauet, Thomas
Hehn, Michel
Mangin, Stéphane
Ciccarelli, Chiara
contents The optical manipulation of magnetism enabled by rare earth-transition metal ferrimagnets holds the promise of ultrafast, energy efficient spintronic technologies. This work investigates laser-induced picosecond spin currents generated by ferrimagnetic GdCo via terahertz emission spectroscopy. A suppression of the THz emission and spin current is observed at magnetization compensation when varying the temperature or alloy composition in the presence of a magnetic field. It is demonstrated that this is due to the formation of domains in the GdCo equilibrium magnetic configuration. Without an applied magnetic field, the picosecond spin current persists at the compensation point. The experimental findings support the model for THz spin current generation based on transport of hot spin-polarized electrons, which is dominated by the Co sublattice at room temperature. Only at low temperature a comparable contribution from Gd is detected but with slower dynamics. Finally, spectral analysis reveals a blueshift of the THz emission related to the formation of magnetic domains close to magnetization compensation.
format Preprint
id arxiv_https___arxiv_org_abs_2409_03088
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Origin of the laser-induced picosecond spin current across magnetization compensation in ferrimagnetic GdCo
Antonio, Guillermo Nava
Remy, Quentin
Lin, Jun-Xiao
Guen, Yann Le
Hamara, Dominik
Compton-Stewart, Jude
Barker, Joseph
Hauet, Thomas
Hehn, Michel
Mangin, Stéphane
Ciccarelli, Chiara
Mesoscale and Nanoscale Physics
Materials Science
Applied Physics
The optical manipulation of magnetism enabled by rare earth-transition metal ferrimagnets holds the promise of ultrafast, energy efficient spintronic technologies. This work investigates laser-induced picosecond spin currents generated by ferrimagnetic GdCo via terahertz emission spectroscopy. A suppression of the THz emission and spin current is observed at magnetization compensation when varying the temperature or alloy composition in the presence of a magnetic field. It is demonstrated that this is due to the formation of domains in the GdCo equilibrium magnetic configuration. Without an applied magnetic field, the picosecond spin current persists at the compensation point. The experimental findings support the model for THz spin current generation based on transport of hot spin-polarized electrons, which is dominated by the Co sublattice at room temperature. Only at low temperature a comparable contribution from Gd is detected but with slower dynamics. Finally, spectral analysis reveals a blueshift of the THz emission related to the formation of magnetic domains close to magnetization compensation.
title Origin of the laser-induced picosecond spin current across magnetization compensation in ferrimagnetic GdCo
topic Mesoscale and Nanoscale Physics
Materials Science
Applied Physics
url https://arxiv.org/abs/2409.03088