Temperature shift of magnetic-field-dependent photoluminescence features of nitrogen-vacancy ensembles in diamond

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Hauptverfasser: Rodzoń, Irena, Zhang, Xue, Ivády, Viktor, Zheng, Huijie, Wickenbrock, Arne, Budker, Dmitry
Format: Preprint
Veröffentlicht: 2024
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author Rodzoń, Irena
Zhang, Xue
Ivády, Viktor
Zheng, Huijie
Wickenbrock, Arne
Budker, Dmitry
author_facet Rodzoń, Irena
Zhang, Xue
Ivády, Viktor
Zheng, Huijie
Wickenbrock, Arne
Budker, Dmitry
contents Recently significant attention has been paid to magnetic-field-dependent photoluminescence (PL) features of the negatively charged nitrogen-vacancy (NV) centers in diamond. These features are used for microwave-free sensing and are indicative of the spin-bath properties in the diamond sample. Examinating the temperature dependence of the PL features allows to identify both temperature dependent and independent features, and to utilize them in diamond-based quantum sensing and dynamic nuclear polarization applications. Here, we study the thermal variability of many different features visible in a wide range of magnetic fields. To this end, we first discuss the origin of the features and tentatively assign the previously unidentified features to cross relaxation of NV center containing multi-spin systems. The experimental results are compared with theoretically predicted temperature shifts deduced from a combination of thermal expansion and electron-phonon interactions. A deeper insight into the thermal behavior of a wide array of the features may come with important consequences for various applications in high-precision NV thermometry, gyroscopes, solid-state clocks, and biomagnetic measurements.
format Preprint
id arxiv_https___arxiv_org_abs_2409_03608
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Temperature shift of magnetic-field-dependent photoluminescence features of nitrogen-vacancy ensembles in diamond
Rodzoń, Irena
Zhang, Xue
Ivády, Viktor
Zheng, Huijie
Wickenbrock, Arne
Budker, Dmitry
Quantum Physics
Applied Physics
Atomic Physics
Recently significant attention has been paid to magnetic-field-dependent photoluminescence (PL) features of the negatively charged nitrogen-vacancy (NV) centers in diamond. These features are used for microwave-free sensing and are indicative of the spin-bath properties in the diamond sample. Examinating the temperature dependence of the PL features allows to identify both temperature dependent and independent features, and to utilize them in diamond-based quantum sensing and dynamic nuclear polarization applications. Here, we study the thermal variability of many different features visible in a wide range of magnetic fields. To this end, we first discuss the origin of the features and tentatively assign the previously unidentified features to cross relaxation of NV center containing multi-spin systems. The experimental results are compared with theoretically predicted temperature shifts deduced from a combination of thermal expansion and electron-phonon interactions. A deeper insight into the thermal behavior of a wide array of the features may come with important consequences for various applications in high-precision NV thermometry, gyroscopes, solid-state clocks, and biomagnetic measurements.
title Temperature shift of magnetic-field-dependent photoluminescence features of nitrogen-vacancy ensembles in diamond
topic Quantum Physics
Applied Physics
Atomic Physics
url https://arxiv.org/abs/2409.03608