Factors influencing quantum evaporation of helium from polar semiconductors from first principles
Fuente:
arXiv
Saved in:
| Main Authors: | , , , , |
|---|---|
| Format: | Preprint |
| Published: |
2024
|
| Subjects: | |
| Online Access: | |
| Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
| _version_ | 1866909307357888512 |
|---|---|
| author | Dheer, Lakshay Tan, Liang Z. Lyon, S. A. Schenkel, Thomas Griffin, Sinéad M. |
| author_facet | Dheer, Lakshay Tan, Liang Z. Lyon, S. A. Schenkel, Thomas Griffin, Sinéad M. |
| contents | While there is much indirect evidence for the existence of dark matter (DM), to date it has evaded detection. Current efforts focus on DM masses over $\sim$GeV -- to push the sensitivity of DM searches to lower masses, new DM targets and detection schemes are needed. In this work, we focus on the latter - a novel detection scheme recently proposed to detect ~10-100 meV phonons in polar target materials. Previous work showed that well-motivated models of DM can interact with polar semiconductors to produce an athermal population of phonons. This new sensing scheme proposes that these phonons then facilitate quantum evaporation of $^3$He from a van der Waals film deposited on the target material. However, a fundamental understanding of the underlying process is still unclear, with several uncertainties related to the precise rate of evaporation and how it can be controlled. In this work, we use \textit{ab initio} density functional theory (DFT) calculations to compare the adsorption energies of helium atoms on a polar target material, sodium iodide (NaI), to understand the underlying evaporation physics. We explore the role of surface termination, monolayer coverage and elemental species on the rate of He evaporation from the target material. Using this, we discuss the optimal target features for He-evaporation experiments and their range of tunability through chemical and physical modifications such as applied field and surface termination. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2409_03857 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Factors influencing quantum evaporation of helium from polar semiconductors from first principles Dheer, Lakshay Tan, Liang Z. Lyon, S. A. Schenkel, Thomas Griffin, Sinéad M. High Energy Physics - Phenomenology Mesoscale and Nanoscale Physics Materials Science Instrumentation and Detectors While there is much indirect evidence for the existence of dark matter (DM), to date it has evaded detection. Current efforts focus on DM masses over $\sim$GeV -- to push the sensitivity of DM searches to lower masses, new DM targets and detection schemes are needed. In this work, we focus on the latter - a novel detection scheme recently proposed to detect ~10-100 meV phonons in polar target materials. Previous work showed that well-motivated models of DM can interact with polar semiconductors to produce an athermal population of phonons. This new sensing scheme proposes that these phonons then facilitate quantum evaporation of $^3$He from a van der Waals film deposited on the target material. However, a fundamental understanding of the underlying process is still unclear, with several uncertainties related to the precise rate of evaporation and how it can be controlled. In this work, we use \textit{ab initio} density functional theory (DFT) calculations to compare the adsorption energies of helium atoms on a polar target material, sodium iodide (NaI), to understand the underlying evaporation physics. We explore the role of surface termination, monolayer coverage and elemental species on the rate of He evaporation from the target material. Using this, we discuss the optimal target features for He-evaporation experiments and their range of tunability through chemical and physical modifications such as applied field and surface termination. |
| title | Factors influencing quantum evaporation of helium from polar semiconductors from first principles |
| topic | High Energy Physics - Phenomenology Mesoscale and Nanoscale Physics Materials Science Instrumentation and Detectors |
| url | https://arxiv.org/abs/2409.03857 |