Correlated Ligand Electrons in the Transition-Metal Oxide SrRuO$_3$

Fuente: arXiv
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Autori principali: Seki, Yuichi, Wakabayashi, Yuki K., Takeda, Takahito, Inagaki, Kohdai, Fujimori, Shin-ichi, Takeda, Yukiharu, Fujimori, Atsushi, Taniyasu, Yoshitaka, Yamamoto, Hideki, Krockenberger, Yoshiharu, Tanaka, Masaaki, Kobayashi, Masaki
Natura: Preprint
Pubblicazione: 2024
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author Seki, Yuichi
Wakabayashi, Yuki K.
Takeda, Takahito
Inagaki, Kohdai
Fujimori, Shin-ichi
Takeda, Yukiharu
Fujimori, Atsushi
Taniyasu, Yoshitaka
Yamamoto, Hideki
Krockenberger, Yoshiharu
Tanaka, Masaaki
Kobayashi, Masaki
author_facet Seki, Yuichi
Wakabayashi, Yuki K.
Takeda, Takahito
Inagaki, Kohdai
Fujimori, Shin-ichi
Takeda, Yukiharu
Fujimori, Atsushi
Taniyasu, Yoshitaka
Yamamoto, Hideki
Krockenberger, Yoshiharu
Tanaka, Masaaki
Kobayashi, Masaki
contents In transition-metal compounds, the transition-metal d electrons play an important role in their physical properties; however, the effects of the electron correlation between the ligand p electrons have not been clear yet. In this Letter, the Ru 4d and O 2p partial density of states (PDOS) in transition-metal oxide SrRuO$_3$ involving Weyl fermions are investigated by resonant photoemission spectroscopy. The observations demonstrate that the O 2p PDOS is distorted from that predicted by first-principles calculations than the Ru 4d PDOS. The results indicate that the electron correlation in the ligand orbitals will be important to understand the electronic structure of the p-d hybridized state in strongly correlated electron systems, even with topological states.
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id arxiv_https___arxiv_org_abs_2409_04062
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Correlated Ligand Electrons in the Transition-Metal Oxide SrRuO$_3$
Seki, Yuichi
Wakabayashi, Yuki K.
Takeda, Takahito
Inagaki, Kohdai
Fujimori, Shin-ichi
Takeda, Yukiharu
Fujimori, Atsushi
Taniyasu, Yoshitaka
Yamamoto, Hideki
Krockenberger, Yoshiharu
Tanaka, Masaaki
Kobayashi, Masaki
Strongly Correlated Electrons
Materials Science
In transition-metal compounds, the transition-metal d electrons play an important role in their physical properties; however, the effects of the electron correlation between the ligand p electrons have not been clear yet. In this Letter, the Ru 4d and O 2p partial density of states (PDOS) in transition-metal oxide SrRuO$_3$ involving Weyl fermions are investigated by resonant photoemission spectroscopy. The observations demonstrate that the O 2p PDOS is distorted from that predicted by first-principles calculations than the Ru 4d PDOS. The results indicate that the electron correlation in the ligand orbitals will be important to understand the electronic structure of the p-d hybridized state in strongly correlated electron systems, even with topological states.
title Correlated Ligand Electrons in the Transition-Metal Oxide SrRuO$_3$
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2409.04062