Large spontaneous Hall effect with flexible domain control in an antiferromagnetic material TaMnP

Fuente: arXiv
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Auteurs principaux: Kotegawa, Hisashi, Nakamura, Akira, Huyen, Vu Thi Ngoc, Arai, Yuki, Tou, Hideki, Sugawara, Hitoshi, Hayashi, Junichi, Takeda, Keiki, Tabata, Chihiro, Kaneko, Koji, Kodama, Katsuaki, Suzuki, Michi-To
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Publié: 2024
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author Kotegawa, Hisashi
Nakamura, Akira
Huyen, Vu Thi Ngoc
Arai, Yuki
Tou, Hideki
Sugawara, Hitoshi
Hayashi, Junichi
Takeda, Keiki
Tabata, Chihiro
Kaneko, Koji
Kodama, Katsuaki
Suzuki, Michi-To
author_facet Kotegawa, Hisashi
Nakamura, Akira
Huyen, Vu Thi Ngoc
Arai, Yuki
Tou, Hideki
Sugawara, Hitoshi
Hayashi, Junichi
Takeda, Keiki
Tabata, Chihiro
Kaneko, Koji
Kodama, Katsuaki
Suzuki, Michi-To
contents Antiferromagnets without parity-time ($\mathcal{PT}$) symmetry offer novel perspectives in the field of functional magnetic materials. Among them, those with ferromagnetic-like responses are promising candidates for future applications such as antiferromagnetic (AF) memory; however, examples showing large effects are extremely limited. In this study, we show that the orthorhombic system TaMnP exhibits a large anomalous Hall conductivity (AHC) $\sim360-370$ $Ω^{-1}$cm$^{-1}$ in spite of the small net magnetization $\sim10^{-2}$ $μ_B$/Mn. Our neutron scattering experiment and the observation of the AH effect indicated that a magnetic structure of TaMnP was dominated by an AF component represented by $B_{3g}$ with the propagation vector $q=0$. Furthermore, we confirmed that the obtained AHC is among the largest observed in AF materials at zero fields. Additionally, our first-principles calculations revealed that the spin-orbit interaction originating in the nonmagnetic Ta-$5d$ electrons significantly contributes to enhancing Berry curvatures in the momentum space. We found that the magnetic fields along all the crystal axes triggered the AF domain switching, indicating the possibility of controlling the AF domain using the small net magnetization, which is symmetrically different.
format Preprint
id arxiv_https___arxiv_org_abs_2409_04064
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Large spontaneous Hall effect with flexible domain control in an antiferromagnetic material TaMnP
Kotegawa, Hisashi
Nakamura, Akira
Huyen, Vu Thi Ngoc
Arai, Yuki
Tou, Hideki
Sugawara, Hitoshi
Hayashi, Junichi
Takeda, Keiki
Tabata, Chihiro
Kaneko, Koji
Kodama, Katsuaki
Suzuki, Michi-To
Strongly Correlated Electrons
Materials Science
Antiferromagnets without parity-time ($\mathcal{PT}$) symmetry offer novel perspectives in the field of functional magnetic materials. Among them, those with ferromagnetic-like responses are promising candidates for future applications such as antiferromagnetic (AF) memory; however, examples showing large effects are extremely limited. In this study, we show that the orthorhombic system TaMnP exhibits a large anomalous Hall conductivity (AHC) $\sim360-370$ $Ω^{-1}$cm$^{-1}$ in spite of the small net magnetization $\sim10^{-2}$ $μ_B$/Mn. Our neutron scattering experiment and the observation of the AH effect indicated that a magnetic structure of TaMnP was dominated by an AF component represented by $B_{3g}$ with the propagation vector $q=0$. Furthermore, we confirmed that the obtained AHC is among the largest observed in AF materials at zero fields. Additionally, our first-principles calculations revealed that the spin-orbit interaction originating in the nonmagnetic Ta-$5d$ electrons significantly contributes to enhancing Berry curvatures in the momentum space. We found that the magnetic fields along all the crystal axes triggered the AF domain switching, indicating the possibility of controlling the AF domain using the small net magnetization, which is symmetrically different.
title Large spontaneous Hall effect with flexible domain control in an antiferromagnetic material TaMnP
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2409.04064