High harmonic spectroscopy reveals anisotropy of the Mott to Charge-Density-Wave phase transition in TiSe$_2$
Fuente:
arXiv
Salvato in:
| Autori principali: | , , , , , , , , , , |
|---|---|
| Natura: | Preprint |
| Pubblicazione: |
2024
|
| Soggetti: | |
| Accesso online: | |
| Tags: |
Aggiungi Tag
Nessun Tag, puoi essere il primo ad aggiungerne!!
|
| _version_ | 1866915611160870912 |
|---|---|
| author | Tyulnev, Igor Zhang, Lin Vamos, Lenard Poborska, Julita Bhattacharya, Utso Chhajlany, Ravindra W. Grass, Tobias Mañas-Valero, Samuel Coronado, Eugenio Lewenstein, Maciej Biegert, Jens |
| author_facet | Tyulnev, Igor Zhang, Lin Vamos, Lenard Poborska, Julita Bhattacharya, Utso Chhajlany, Ravindra W. Grass, Tobias Mañas-Valero, Samuel Coronado, Eugenio Lewenstein, Maciej Biegert, Jens |
| contents | This work explores the use of polarization-resolved high harmonic generation (HHG) spectroscopy to investigate the quantum phases and transitions in the correlated charge density wave (CDW) phase of TiSe$_2$. Unlike previous studies focusing on crystallographic changes, the research examines the reordering that occurs within the CDW phase as the material is cooled from room temperature to 14 K. By linking ultrafast field-driven dynamics to the material's potential landscape, the study demonstrates how HHG is sensitive to quantum phase transitions. The findings reveal an anisotropic component below the CDW transition temperature, providing new insights into the nature of this phase. The investigation highlights the interplay between linear and nonlinear optical responses and their departure from simple perturbative dynamics, offering a fresh perspective on correlated quantum phases in condensed matter systems. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2409_04216 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | High harmonic spectroscopy reveals anisotropy of the Mott to Charge-Density-Wave phase transition in TiSe$_2$ Tyulnev, Igor Zhang, Lin Vamos, Lenard Poborska, Julita Bhattacharya, Utso Chhajlany, Ravindra W. Grass, Tobias Mañas-Valero, Samuel Coronado, Eugenio Lewenstein, Maciej Biegert, Jens Strongly Correlated Electrons Materials Science Optics This work explores the use of polarization-resolved high harmonic generation (HHG) spectroscopy to investigate the quantum phases and transitions in the correlated charge density wave (CDW) phase of TiSe$_2$. Unlike previous studies focusing on crystallographic changes, the research examines the reordering that occurs within the CDW phase as the material is cooled from room temperature to 14 K. By linking ultrafast field-driven dynamics to the material's potential landscape, the study demonstrates how HHG is sensitive to quantum phase transitions. The findings reveal an anisotropic component below the CDW transition temperature, providing new insights into the nature of this phase. The investigation highlights the interplay between linear and nonlinear optical responses and their departure from simple perturbative dynamics, offering a fresh perspective on correlated quantum phases in condensed matter systems. |
| title | High harmonic spectroscopy reveals anisotropy of the Mott to Charge-Density-Wave phase transition in TiSe$_2$ |
| topic | Strongly Correlated Electrons Materials Science Optics |
| url | https://arxiv.org/abs/2409.04216 |