Enhanced magnetic dichroism in darkfield UV photoemission electron microscopy

Fuente: arXiv
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Main Authors: Paleschke, Maximilian, Huber, David, Wührl, Friederike, Chiang, Cheng-Tien, Schumann, Frank O., Henk, Jürgen, Widdra, Wolf
Format: Preprint
Published: 2024
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_version_ 1866910945947680768
author Paleschke, Maximilian
Huber, David
Wührl, Friederike
Chiang, Cheng-Tien
Schumann, Frank O.
Henk, Jürgen
Widdra, Wolf
author_facet Paleschke, Maximilian
Huber, David
Wührl, Friederike
Chiang, Cheng-Tien
Schumann, Frank O.
Henk, Jürgen
Widdra, Wolf
contents Photoemission electron microscopy (PEEM) has evolved into an indispensable tool for structural and magnetic characterization of surfaces at the nanometer scale. In strong contrast to synchrotron-radiation-based X-ray PEEM as a leading method for element-specific magnetic properties via magnetic circular dichroism (MCD), laboratory ultraviolet (UV) PEEM has seen limited application with much smaller dichroism effects for in-plane magnetization. Here we introduce darkfield PEEM as a novel approach to enhance MCD contrast in threshold photoemission, enabling efficient MCD imaging with significantly enhanced contrast by an order-of-magnitude for Fe(001). This advancement paves the way for MCD imaging on femtosecond timescales using modern lasers. The experimental results will be quantitatively benchmarked against advanced relativistic photoemission calculations.
format Preprint
id arxiv_https___arxiv_org_abs_2409_04771
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Enhanced magnetic dichroism in darkfield UV photoemission electron microscopy
Paleschke, Maximilian
Huber, David
Wührl, Friederike
Chiang, Cheng-Tien
Schumann, Frank O.
Henk, Jürgen
Widdra, Wolf
Materials Science
Mesoscale and Nanoscale Physics
Photoemission electron microscopy (PEEM) has evolved into an indispensable tool for structural and magnetic characterization of surfaces at the nanometer scale. In strong contrast to synchrotron-radiation-based X-ray PEEM as a leading method for element-specific magnetic properties via magnetic circular dichroism (MCD), laboratory ultraviolet (UV) PEEM has seen limited application with much smaller dichroism effects for in-plane magnetization. Here we introduce darkfield PEEM as a novel approach to enhance MCD contrast in threshold photoemission, enabling efficient MCD imaging with significantly enhanced contrast by an order-of-magnitude for Fe(001). This advancement paves the way for MCD imaging on femtosecond timescales using modern lasers. The experimental results will be quantitatively benchmarked against advanced relativistic photoemission calculations.
title Enhanced magnetic dichroism in darkfield UV photoemission electron microscopy
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2409.04771