Ferroelectric tuning of the valley polarized metal-semiconductor transition in Mn2P2S3Se3/Sc2CO2 van der Waals heterostructures and application to nonlinear Hall effect devices

Fuente: arXiv
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Auteurs principaux: Sun, Hanbo, Ren, Yewei, Wu, Chao, Dong, Pengqiang, Zhang, Weixi, Wu, Yin-Zhong, Li, Ping
Format: Preprint
Publié: 2024
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author Sun, Hanbo
Ren, Yewei
Wu, Chao
Dong, Pengqiang
Zhang, Weixi
Wu, Yin-Zhong
Li, Ping
author_facet Sun, Hanbo
Ren, Yewei
Wu, Chao
Dong, Pengqiang
Zhang, Weixi
Wu, Yin-Zhong
Li, Ping
contents In order to promote the development of the next generation of nano-spintronic devices, it is of great significance to tune the freedom of valley in two-dimensional (2D) materials. Here, we propose a mechanism for manipulating the valley and nonlinear Hall effect by the 2D ferroelectric substrate. The monolayer Mn2P2S3Se3 is a robust antiferromagnetic valley polarized semiconductor. Importantly, the valley polarized metal-semiconductor phase transition of Mn2P2S3Se3 can be effectively tuned by switching the ferroelectric polarization of Sc2CO2. We reveal the microscopic mechanism of phase transition, which origins from the charge transfer and band alignment. Additionally, we find that transformed polarization direction of Sc2CO2 flexibly manipulate the Berry curvature dipole. Based on this discovery, we present the detection valley polarized metal-semiconductor transition by the nonlinear Hall effect devices. These findings not only offer a scheme to tune the valley degree of freedom, but also provide promising platform to design the nonlinear Hall effect devices.
format Preprint
id arxiv_https___arxiv_org_abs_2409_06181
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Ferroelectric tuning of the valley polarized metal-semiconductor transition in Mn2P2S3Se3/Sc2CO2 van der Waals heterostructures and application to nonlinear Hall effect devices
Sun, Hanbo
Ren, Yewei
Wu, Chao
Dong, Pengqiang
Zhang, Weixi
Wu, Yin-Zhong
Li, Ping
Materials Science
Mesoscale and Nanoscale Physics
In order to promote the development of the next generation of nano-spintronic devices, it is of great significance to tune the freedom of valley in two-dimensional (2D) materials. Here, we propose a mechanism for manipulating the valley and nonlinear Hall effect by the 2D ferroelectric substrate. The monolayer Mn2P2S3Se3 is a robust antiferromagnetic valley polarized semiconductor. Importantly, the valley polarized metal-semiconductor phase transition of Mn2P2S3Se3 can be effectively tuned by switching the ferroelectric polarization of Sc2CO2. We reveal the microscopic mechanism of phase transition, which origins from the charge transfer and band alignment. Additionally, we find that transformed polarization direction of Sc2CO2 flexibly manipulate the Berry curvature dipole. Based on this discovery, we present the detection valley polarized metal-semiconductor transition by the nonlinear Hall effect devices. These findings not only offer a scheme to tune the valley degree of freedom, but also provide promising platform to design the nonlinear Hall effect devices.
title Ferroelectric tuning of the valley polarized metal-semiconductor transition in Mn2P2S3Se3/Sc2CO2 van der Waals heterostructures and application to nonlinear Hall effect devices
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2409.06181