Time Crystals from single-molecule magnet arrays

Fuente: arXiv
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Autores principales: Sarkar, Subhajit, Dubi, Yonatan
Formato: Preprint
Publicado: 2024
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author Sarkar, Subhajit
Dubi, Yonatan
author_facet Sarkar, Subhajit
Dubi, Yonatan
contents Time crystals, a unique non-equilibrium quantum phenomenon with promising applications in current quantum technologies, mark a significant advance in quantum mechanics. Although traditionally studied in atom-cavity and optical lattice systems, pursuing alternative nanoscale platforms for time crystals is crucial. Here we theoretically predict discrete time-crystals in a periodically driven molecular magnet array, modeled by a spin-S Heisenberg Hamiltonian with significant quadratic anisotropy, taken with realistic and experimentally relevant physical parameters. Surprisingly, we find that the time-crystal response frequency correlates with the energy levels of the individual magnets and is essentially independent of the exchange coupling. The latter is unexpectedly manifested through a pulse-like oscillation in the magnetization envelope, signaling a many-body response. These results show that molecular magnets can be a rich platform for studying time-crystalline behavior and possibly other out-of-equilibrium quantum many-body dynamics.
format Preprint
id arxiv_https___arxiv_org_abs_2409_10816
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Time Crystals from single-molecule magnet arrays
Sarkar, Subhajit
Dubi, Yonatan
Quantum Physics
Mesoscale and Nanoscale Physics
Statistical Mechanics
Strongly Correlated Electrons
Time crystals, a unique non-equilibrium quantum phenomenon with promising applications in current quantum technologies, mark a significant advance in quantum mechanics. Although traditionally studied in atom-cavity and optical lattice systems, pursuing alternative nanoscale platforms for time crystals is crucial. Here we theoretically predict discrete time-crystals in a periodically driven molecular magnet array, modeled by a spin-S Heisenberg Hamiltonian with significant quadratic anisotropy, taken with realistic and experimentally relevant physical parameters. Surprisingly, we find that the time-crystal response frequency correlates with the energy levels of the individual magnets and is essentially independent of the exchange coupling. The latter is unexpectedly manifested through a pulse-like oscillation in the magnetization envelope, signaling a many-body response. These results show that molecular magnets can be a rich platform for studying time-crystalline behavior and possibly other out-of-equilibrium quantum many-body dynamics.
title Time Crystals from single-molecule magnet arrays
topic Quantum Physics
Mesoscale and Nanoscale Physics
Statistical Mechanics
Strongly Correlated Electrons
url https://arxiv.org/abs/2409.10816