Saved in:
Bibliographic Details
Main Authors: Grimsley, Harper R., Evangelista, Francesco A.
Format: Preprint
Published: 2024
Subjects:
Online Access:https://arxiv.org/abs/2409.11210
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866929662767136768
author Grimsley, Harper R.
Evangelista, Francesco A.
author_facet Grimsley, Harper R.
Evangelista, Francesco A.
contents The prediction of electronic structure for strongly correlated molecules represents a promising application for near-term quantum computers. Significant attention has been paid to ground state wavefunctions, but excited states of molecules are relatively unexplored. In this work, we consider the ADAPT-VQE algorithm, a single-reference approach for obtaining ground states, and its state-averaged generalization for computing multiple states at once. We demonstrate for both rectangular and linear H$_4$, as well as for BeH$_2$, that this approach, which we call MORE-ADAPT-VQE, can make better use of small excitation manifolds than an analagous method based on a single-reference ADAPT-VQE calculation, q-sc-EOM. In particular, MORE-ADAPT-VQE is able to accurately describe both avoided crossings and crossings between states of different symmetries. In addition to more accurate excited state energies, MORE-ADAPT-VQE can recover accurate transition dipole moments in situations where traditional ADAPT-VQE and q-sc-EOM struggle. These improvements suggest a promising direction toward the use of quantum computers for difficult excited state problems.
format Preprint
id arxiv_https___arxiv_org_abs_2409_11210
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Challenging Excited States from Adaptive Quantum Eigensolvers: Subspace Expansions vs. State-Averaged Strategies
Grimsley, Harper R.
Evangelista, Francesco A.
Quantum Physics
The prediction of electronic structure for strongly correlated molecules represents a promising application for near-term quantum computers. Significant attention has been paid to ground state wavefunctions, but excited states of molecules are relatively unexplored. In this work, we consider the ADAPT-VQE algorithm, a single-reference approach for obtaining ground states, and its state-averaged generalization for computing multiple states at once. We demonstrate for both rectangular and linear H$_4$, as well as for BeH$_2$, that this approach, which we call MORE-ADAPT-VQE, can make better use of small excitation manifolds than an analagous method based on a single-reference ADAPT-VQE calculation, q-sc-EOM. In particular, MORE-ADAPT-VQE is able to accurately describe both avoided crossings and crossings between states of different symmetries. In addition to more accurate excited state energies, MORE-ADAPT-VQE can recover accurate transition dipole moments in situations where traditional ADAPT-VQE and q-sc-EOM struggle. These improvements suggest a promising direction toward the use of quantum computers for difficult excited state problems.
title Challenging Excited States from Adaptive Quantum Eigensolvers: Subspace Expansions vs. State-Averaged Strategies
topic Quantum Physics
url https://arxiv.org/abs/2409.11210