Origin of the non-Fermi-liquid behavior in CeRh2As2

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Main Authors: Khanenko, P., Hafner, D., Semeniuk, K., Banda, J., Luehmann, T., Baertl, F., Kotte, T., Wosnitza, J., Zwicknagl, G., Geibel, C., Landaeta, J. F., Khim, S., Hassinger, E., Brando, M.
Format: Preprint
Published: 2024
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author Khanenko, P.
Hafner, D.
Semeniuk, K.
Banda, J.
Luehmann, T.
Baertl, F.
Kotte, T.
Wosnitza, J.
Zwicknagl, G.
Geibel, C.
Landaeta, J. F.
Khim, S.
Hassinger, E.
Brando, M.
author_facet Khanenko, P.
Hafner, D.
Semeniuk, K.
Banda, J.
Luehmann, T.
Baertl, F.
Kotte, T.
Wosnitza, J.
Zwicknagl, G.
Geibel, C.
Landaeta, J. F.
Khim, S.
Hassinger, E.
Brando, M.
contents Unconventional superconductivity in heavy-fermion systems appears often near magnetic quantum critical points (QCPs). This seems to be the case also for CeRh2As2 (Tc $\approx$ 0.31 K). CeRh2As2 shows two superconducting (SC) phases, SC1 and SC2, for a magnetic field along the c axis of the tetragonal unit cell, but only the SC1 phase is observed for a field along the basal plane. Furthermore, another ordered state (phase-I) is observed below T0 $\approx$ 0.48 K whose nature is still unclear: Thermodynamic and magnetic measurements pointed to a non magnetic multipolar state, but recent $μ$SR and NQR/NMR experiments have clearly detected antiferromagnetic (AFM) order below T0 . Also, quasi-two-dimensional AFM fluctuations were observed in NMR and neutron-scattering experiments above T0. The proximity of a QCP is indicated by non-Fermi-liquid (NFL) behavior observed above the ordered states in both specific heat $C(T)/T \propto T^{-0.6}$ and resistivity $ρ(T) \propto T^{0.5}$. These T-dependencies are not compatible with any generic AFM QCP. Because of the strong magnetic-field anisotropy of both the SC phase and phase I, it is possible to study a field-induced SC QCP as well a phase-I QCP by varying the angle $α$ between the field and the c axis. Thus, by examining the behavior of the electronic specific-heat coefficient C(T)/T across these QCPs, we can determine which phase is associated with the NFL behavior. Here, we present low-temperature specific-heat measurements taken in a magnetic field as high as 21 T applied at several angles $α$. We observe that the NFL behavior does very weakly depend on the field and on the angle $α$, a result that is at odd with that observations in standard magnetic QCPs. This suggests a nonmagnetic origin of the quantum critical fluctuations.
format Preprint
id arxiv_https___arxiv_org_abs_2409_11894
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Origin of the non-Fermi-liquid behavior in CeRh2As2
Khanenko, P.
Hafner, D.
Semeniuk, K.
Banda, J.
Luehmann, T.
Baertl, F.
Kotte, T.
Wosnitza, J.
Zwicknagl, G.
Geibel, C.
Landaeta, J. F.
Khim, S.
Hassinger, E.
Brando, M.
Strongly Correlated Electrons
Unconventional superconductivity in heavy-fermion systems appears often near magnetic quantum critical points (QCPs). This seems to be the case also for CeRh2As2 (Tc $\approx$ 0.31 K). CeRh2As2 shows two superconducting (SC) phases, SC1 and SC2, for a magnetic field along the c axis of the tetragonal unit cell, but only the SC1 phase is observed for a field along the basal plane. Furthermore, another ordered state (phase-I) is observed below T0 $\approx$ 0.48 K whose nature is still unclear: Thermodynamic and magnetic measurements pointed to a non magnetic multipolar state, but recent $μ$SR and NQR/NMR experiments have clearly detected antiferromagnetic (AFM) order below T0 . Also, quasi-two-dimensional AFM fluctuations were observed in NMR and neutron-scattering experiments above T0. The proximity of a QCP is indicated by non-Fermi-liquid (NFL) behavior observed above the ordered states in both specific heat $C(T)/T \propto T^{-0.6}$ and resistivity $ρ(T) \propto T^{0.5}$. These T-dependencies are not compatible with any generic AFM QCP. Because of the strong magnetic-field anisotropy of both the SC phase and phase I, it is possible to study a field-induced SC QCP as well a phase-I QCP by varying the angle $α$ between the field and the c axis. Thus, by examining the behavior of the electronic specific-heat coefficient C(T)/T across these QCPs, we can determine which phase is associated with the NFL behavior. Here, we present low-temperature specific-heat measurements taken in a magnetic field as high as 21 T applied at several angles $α$. We observe that the NFL behavior does very weakly depend on the field and on the angle $α$, a result that is at odd with that observations in standard magnetic QCPs. This suggests a nonmagnetic origin of the quantum critical fluctuations.
title Origin of the non-Fermi-liquid behavior in CeRh2As2
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2409.11894