Revealing the Geometrical and Vibrational Properties of the Defects Driving the Boson Peak
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arXiv
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| Format: | Preprint |
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2024
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| _version_ | 1866908582468911104 |
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| author | Mahajan, Shivam Han, Darryl Seow Yang Jiang, Cunyuan Baggioli, Matteo Ciamarra, Massimo Pica |
| author_facet | Mahajan, Shivam Han, Darryl Seow Yang Jiang, Cunyuan Baggioli, Matteo Ciamarra, Massimo Pica |
| contents | In amorphous solids, the vibrational density of states shows an excess of modes over the Debye model, known as the boson peak, whose origin remains unclear. Studies suggest a link to quasi-localized nonphononic vibrations or 'defects,' but identifying them is challenging due to hybridization with phonons that renders methods based on localization properties, such as the participation ratio, unreliable. We introduce a practical method to separate hybridized phonons from localized vibrations and find that boson peak phonons hybridize with compact, two-dimensional defects exhibiting oscillatory pure shear deformations. These two-dimensional defects are also exposed by the procedure recently employed to identify stringlets (Nature Physics volume 18, pages 669-677 (2022)), suggesting that these may not be one-dimensional objects as speculated. Our work demonstrates the presence of localized defects at the boson peak frequency and provides a comprehensive characterization of their vibrational and geometric properties, resolving the tension between the concepts of quasi-localized quadrupolar defects and stringlets. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2409_13169 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Revealing the Geometrical and Vibrational Properties of the Defects Driving the Boson Peak Mahajan, Shivam Han, Darryl Seow Yang Jiang, Cunyuan Baggioli, Matteo Ciamarra, Massimo Pica Soft Condensed Matter In amorphous solids, the vibrational density of states shows an excess of modes over the Debye model, known as the boson peak, whose origin remains unclear. Studies suggest a link to quasi-localized nonphononic vibrations or 'defects,' but identifying them is challenging due to hybridization with phonons that renders methods based on localization properties, such as the participation ratio, unreliable. We introduce a practical method to separate hybridized phonons from localized vibrations and find that boson peak phonons hybridize with compact, two-dimensional defects exhibiting oscillatory pure shear deformations. These two-dimensional defects are also exposed by the procedure recently employed to identify stringlets (Nature Physics volume 18, pages 669-677 (2022)), suggesting that these may not be one-dimensional objects as speculated. Our work demonstrates the presence of localized defects at the boson peak frequency and provides a comprehensive characterization of their vibrational and geometric properties, resolving the tension between the concepts of quasi-localized quadrupolar defects and stringlets. |
| title | Revealing the Geometrical and Vibrational Properties of the Defects Driving the Boson Peak |
| topic | Soft Condensed Matter |
| url | https://arxiv.org/abs/2409.13169 |