Windmill droplets. Optically induced rotation of biphase oil-in-water droplets

Fuente: arXiv
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Autori principali: del Pozo, Jesús J., Bonhome-Espinosa, Ana B., Sun, Wei, Gutiérrez-Ariza, Carlos, Rica, Raúl A., Rodríguez-Arco, Laura
Natura: Preprint
Pubblicazione: 2024
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author del Pozo, Jesús J.
Bonhome-Espinosa, Ana B.
Sun, Wei
Gutiérrez-Ariza, Carlos
Rica, Raúl A.
Rodríguez-Arco, Laura
author_facet del Pozo, Jesús J.
Bonhome-Espinosa, Ana B.
Sun, Wei
Gutiérrez-Ariza, Carlos
Rica, Raúl A.
Rodríguez-Arco, Laura
contents In the field of microdroplet manipulation, optical tweezers have been used to form and grow droplets, to transport them, or to measure forces between droplet pairs. However, the exploration of out-of-equilibrium phenomena in optically trapped droplets remains largely uncharted. Here, we report the rotation of biphasic droplets fabricated by co-emulsifying two immiscible liquids (i.e., hydrocarbon and fluorocarbon oils) with a refractive index mismatch in water. When trapped, droplets of a specific geometry rotate around the axis of the laser beam, in what appears to be a dissipative, out-of-equilibrium phenomenon. The rotational frequency, obtained from image analysis is stable and proportional to the beam power. Remarkably, droplets that do not interact with the trapping beam can also be rotated indirectly. This is achieved by positioning the droplets at the center of a circular arrangement of multiple, sequentially activated traps. In this case, the droplet orients towards the location of the active trap by a mechanism yet to be understood. Altogether, our results demonstrate out-from-equilibrium phenomenology in optically trapped biphase droplets, which could inspire the development of devices based on them (e.g., optically induced mixing, etc.). In addition, they may shed light on fundamental principles of optical manipulation of asymmetric particles.
format Preprint
id arxiv_https___arxiv_org_abs_2409_18539
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Windmill droplets. Optically induced rotation of biphase oil-in-water droplets
del Pozo, Jesús J.
Bonhome-Espinosa, Ana B.
Sun, Wei
Gutiérrez-Ariza, Carlos
Rica, Raúl A.
Rodríguez-Arco, Laura
Soft Condensed Matter
Applied Physics
Optics
In the field of microdroplet manipulation, optical tweezers have been used to form and grow droplets, to transport them, or to measure forces between droplet pairs. However, the exploration of out-of-equilibrium phenomena in optically trapped droplets remains largely uncharted. Here, we report the rotation of biphasic droplets fabricated by co-emulsifying two immiscible liquids (i.e., hydrocarbon and fluorocarbon oils) with a refractive index mismatch in water. When trapped, droplets of a specific geometry rotate around the axis of the laser beam, in what appears to be a dissipative, out-of-equilibrium phenomenon. The rotational frequency, obtained from image analysis is stable and proportional to the beam power. Remarkably, droplets that do not interact with the trapping beam can also be rotated indirectly. This is achieved by positioning the droplets at the center of a circular arrangement of multiple, sequentially activated traps. In this case, the droplet orients towards the location of the active trap by a mechanism yet to be understood. Altogether, our results demonstrate out-from-equilibrium phenomenology in optically trapped biphase droplets, which could inspire the development of devices based on them (e.g., optically induced mixing, etc.). In addition, they may shed light on fundamental principles of optical manipulation of asymmetric particles.
title Windmill droplets. Optically induced rotation of biphase oil-in-water droplets
topic Soft Condensed Matter
Applied Physics
Optics
url https://arxiv.org/abs/2409.18539