Helium atom micro-diffraction as a characterisation tool for 2D materials

Fuente: arXiv
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Main Authors: von Jeinsen, Nick, Radic, Aleksandar, Wang, Ke, Zhao, Chenyang, Perez, Vivian, Zhu, Yiru, Chhowalla, Manish, Jardine, Andrew, Ward, David, Lambrick, Sam
Format: Preprint
Published: 2024
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author von Jeinsen, Nick
Radic, Aleksandar
Wang, Ke
Zhao, Chenyang
Perez, Vivian
Zhu, Yiru
Chhowalla, Manish
Jardine, Andrew
Ward, David
Lambrick, Sam
author_facet von Jeinsen, Nick
Radic, Aleksandar
Wang, Ke
Zhao, Chenyang
Perez, Vivian
Zhu, Yiru
Chhowalla, Manish
Jardine, Andrew
Ward, David
Lambrick, Sam
contents We present helium atom micro-diffraction as an ideal technique for characterization of 2D materials due to its ultimate surface sensitivity combined with sub-micron spatial resolution. Thermal energy neutral helium scatters from the valence electron density, 2-3A above the ionic cores of a surface, making the technique ideal for studying 2D materials, where other approaches can struggle due to small interaction cross-sections with few-layer samples. Sub-micron spatial resolution is key development in neutral atom scattering to allow measurements from device-scale samples. We present measurements of monolayer-substrate interactions, thermal expansion coefficients, the electron-phonon coupling constant and vacancy-type defect density on monolayer-MoS2. We also discuss extensions to the presented methods which can be immediately implemented on existing instruments to perform spatial mapping of these material properties.
format Preprint
id arxiv_https___arxiv_org_abs_2409_20461
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Helium atom micro-diffraction as a characterisation tool for 2D materials
von Jeinsen, Nick
Radic, Aleksandar
Wang, Ke
Zhao, Chenyang
Perez, Vivian
Zhu, Yiru
Chhowalla, Manish
Jardine, Andrew
Ward, David
Lambrick, Sam
Applied Physics
Materials Science
We present helium atom micro-diffraction as an ideal technique for characterization of 2D materials due to its ultimate surface sensitivity combined with sub-micron spatial resolution. Thermal energy neutral helium scatters from the valence electron density, 2-3A above the ionic cores of a surface, making the technique ideal for studying 2D materials, where other approaches can struggle due to small interaction cross-sections with few-layer samples. Sub-micron spatial resolution is key development in neutral atom scattering to allow measurements from device-scale samples. We present measurements of monolayer-substrate interactions, thermal expansion coefficients, the electron-phonon coupling constant and vacancy-type defect density on monolayer-MoS2. We also discuss extensions to the presented methods which can be immediately implemented on existing instruments to perform spatial mapping of these material properties.
title Helium atom micro-diffraction as a characterisation tool for 2D materials
topic Applied Physics
Materials Science
url https://arxiv.org/abs/2409.20461