Interband spectroscopy of Landau levels and magnetoexcitons in bulk black phosphorus

Fuente: arXiv
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Autores principales: Okamura, H., Iguchi, S., Sasaki, T., Ikemoto, Y., Moriwaki, T., Akahama, Y.
Formato: Preprint
Publicado: 2024
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author Okamura, H.
Iguchi, S.
Sasaki, T.
Ikemoto, Y.
Moriwaki, T.
Akahama, Y.
author_facet Okamura, H.
Iguchi, S.
Sasaki, T.
Ikemoto, Y.
Moriwaki, T.
Akahama, Y.
contents Low-dimensional systems based on black phosphorus (BP) have recently attracted much interest. Since the crystal structure of BP consists of 2D layers with a strong in-plane anisotropy, its electronic properties at a high magnetic field ($B$) are quite interesting. Here, we report a magneto-optical study of bulk BP at high $B$ to 12 T perpendicular to the 2D layers. In the obtained optical conductivity spectra, periodic peaks are clearly observed corresponding to Landau levels of up to $n$=6 quantum number. They exhibit almost linear shifts with $B$, and from their analysis an electron-hole reduced mass of 0.13 $m_0$ is obtained, where $m_0$ is the electron mass. Many of the peaks appear in pairs, which is interpreted in terms of Zeeman splitting and an electron-hole combined $g$-factor of 6.6 is obtained. In addition, magnetoexciton peaks are observed to shift quadratically with $B$, and the exciton binding energy at $B$=0 is estimated to be 9.7 meV.
format Preprint
id arxiv_https___arxiv_org_abs_2410_04019
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Interband spectroscopy of Landau levels and magnetoexcitons in bulk black phosphorus
Okamura, H.
Iguchi, S.
Sasaki, T.
Ikemoto, Y.
Moriwaki, T.
Akahama, Y.
Mesoscale and Nanoscale Physics
Low-dimensional systems based on black phosphorus (BP) have recently attracted much interest. Since the crystal structure of BP consists of 2D layers with a strong in-plane anisotropy, its electronic properties at a high magnetic field ($B$) are quite interesting. Here, we report a magneto-optical study of bulk BP at high $B$ to 12 T perpendicular to the 2D layers. In the obtained optical conductivity spectra, periodic peaks are clearly observed corresponding to Landau levels of up to $n$=6 quantum number. They exhibit almost linear shifts with $B$, and from their analysis an electron-hole reduced mass of 0.13 $m_0$ is obtained, where $m_0$ is the electron mass. Many of the peaks appear in pairs, which is interpreted in terms of Zeeman splitting and an electron-hole combined $g$-factor of 6.6 is obtained. In addition, magnetoexciton peaks are observed to shift quadratically with $B$, and the exciton binding energy at $B$=0 is estimated to be 9.7 meV.
title Interband spectroscopy of Landau levels and magnetoexcitons in bulk black phosphorus
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2410.04019