Magnetic structure of the noncentrosymmetric magnet Sr2MnSi2O7 through irreducible representation and magnetic space group analyses

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Main Authors: Nambu, Y., Kawamata, M., Pang, X., Murakawa, H., Avdeev, M., Kimura, H., Masuda, H., Hanasaki, N., Onose, Y.
Format: Preprint
Published: 2024
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author Nambu, Y.
Kawamata, M.
Pang, X.
Murakawa, H.
Avdeev, M.
Kimura, H.
Masuda, H.
Hanasaki, N.
Onose, Y.
author_facet Nambu, Y.
Kawamata, M.
Pang, X.
Murakawa, H.
Avdeev, M.
Kimura, H.
Masuda, H.
Hanasaki, N.
Onose, Y.
contents Magnetic structures of the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were examined through neutron diffraction for powder and single-crystalline samples, as well as magnetometry measurements. All allowed magnetic structures under the space group $P\bar{4}2_1 m$ with the magnetic wavevector $\vec{q}_{\rm m}=(0,0,1/2)$~r.l.u., were analysed via irreducible representation and magnetic space group approaches. The compound is refined to have in-plane magnetic moments within the magnetic space group $Cmc2_1.1^{\prime}_c$ (\#36.177) under zero field, which can be altered to $P2_1 2_1 2_1.1^{\prime}_c$ (\#19.28) above $μ_0 H=0.067(5)$~T to align induced weak-ferromagnetic components within one layer on the $ab$-plane. All refined parameters are provided following the recent framework based upon the magnetic space group, which better conveys when exchanging crystallographic information for commensurate magnetic structures.
format Preprint
id arxiv_https___arxiv_org_abs_2410_04042
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Magnetic structure of the noncentrosymmetric magnet Sr2MnSi2O7 through irreducible representation and magnetic space group analyses
Nambu, Y.
Kawamata, M.
Pang, X.
Murakawa, H.
Avdeev, M.
Kimura, H.
Masuda, H.
Hanasaki, N.
Onose, Y.
Strongly Correlated Electrons
Materials Science
Magnetic structures of the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were examined through neutron diffraction for powder and single-crystalline samples, as well as magnetometry measurements. All allowed magnetic structures under the space group $P\bar{4}2_1 m$ with the magnetic wavevector $\vec{q}_{\rm m}=(0,0,1/2)$~r.l.u., were analysed via irreducible representation and magnetic space group approaches. The compound is refined to have in-plane magnetic moments within the magnetic space group $Cmc2_1.1^{\prime}_c$ (\#36.177) under zero field, which can be altered to $P2_1 2_1 2_1.1^{\prime}_c$ (\#19.28) above $μ_0 H=0.067(5)$~T to align induced weak-ferromagnetic components within one layer on the $ab$-plane. All refined parameters are provided following the recent framework based upon the magnetic space group, which better conveys when exchanging crystallographic information for commensurate magnetic structures.
title Magnetic structure of the noncentrosymmetric magnet Sr2MnSi2O7 through irreducible representation and magnetic space group analyses
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2410.04042