Observation of the spiral spin liquid in a triangular-lattice material

Fuente: arXiv
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Auteurs principaux: Andriushin, N. D., Nikitin, S. E., Fjellvåg, Ø. S., White, J. S., Podlesnyak, A., Inosov, D. S., Rahn, M. C., Schmidt, M., Baenitz, M., Sukhanov, A. S.
Format: Preprint
Publié: 2024
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author Andriushin, N. D.
Nikitin, S. E.
Fjellvåg, Ø. S.
White, J. S.
Podlesnyak, A.
Inosov, D. S.
Rahn, M. C.
Schmidt, M.
Baenitz, M.
Sukhanov, A. S.
author_facet Andriushin, N. D.
Nikitin, S. E.
Fjellvåg, Ø. S.
White, J. S.
Podlesnyak, A.
Inosov, D. S.
Rahn, M. C.
Schmidt, M.
Baenitz, M.
Sukhanov, A. S.
contents The spiral spin liquid (SSL) is a highly degenerate state characterized by a continuous contour or surface in reciprocal space spanned by a spiral propagation vector. Although the SSL state has been predicted in a number of various theoretical models, very few materials are so far experimentally identified to host such a state. Via combined single-crystal wide-angle and small-angle neutron scattering, we report observation of the SSL in the quasi-two-dimensional delafossite AgCrSe$_2$. We show that it is a very close realization of the ideal Heisenberg $J_1$--$J_2$--$J_3$ frustrated model on the triangular lattice. By supplementing our experimental results with microscopic spin-dynamics simulations, we demonstrate how such exotic magnetic states are driven by thermal fluctuations and exchange frustration.
format Preprint
id arxiv_https___arxiv_org_abs_2410_04954
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Observation of the spiral spin liquid in a triangular-lattice material
Andriushin, N. D.
Nikitin, S. E.
Fjellvåg, Ø. S.
White, J. S.
Podlesnyak, A.
Inosov, D. S.
Rahn, M. C.
Schmidt, M.
Baenitz, M.
Sukhanov, A. S.
Strongly Correlated Electrons
The spiral spin liquid (SSL) is a highly degenerate state characterized by a continuous contour or surface in reciprocal space spanned by a spiral propagation vector. Although the SSL state has been predicted in a number of various theoretical models, very few materials are so far experimentally identified to host such a state. Via combined single-crystal wide-angle and small-angle neutron scattering, we report observation of the SSL in the quasi-two-dimensional delafossite AgCrSe$_2$. We show that it is a very close realization of the ideal Heisenberg $J_1$--$J_2$--$J_3$ frustrated model on the triangular lattice. By supplementing our experimental results with microscopic spin-dynamics simulations, we demonstrate how such exotic magnetic states are driven by thermal fluctuations and exchange frustration.
title Observation of the spiral spin liquid in a triangular-lattice material
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2410.04954