Kondo Impurities at a Finite Concentration of Impurities

Fuente: arXiv
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Main Author: Goldstein, Garry
Format: Preprint
Published: 2024
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author Goldstein, Garry
author_facet Goldstein, Garry
contents In this work we study the Kondo impurity problem - at a finite concentration of impurities. We identify two parameter regimes for the Kondo impurity problem. 1) The single impurity limit, where the concentration of Kondo impurities is so low that the background scattering mechanisms (non-magnetic impurities, Umklapp scattering, etc.) of the metal considered are the dominant conduction electron scattering mechanisms at zero temperature. 2) The dilute impurity system limit where the concentration of magnetic impurities is such that they form the dominant mechanism of conduction electron scattering at zero temperature of the metal in question (this is accompanied by a variety of easily detectable Kondo signatures (resistance minimum, specific heat measurements, magnetization as a function of external magnetic field, conduction electron dephasing rates as well as ARPES, RIXS and NMR spectroscopies)) while still being very dilute. Most theoretical efforts are currently in regime where a single isolated impurity is considered - regime 1) while most experimental efforts are in regime 2). We present analytical evidence that this explains the well known discrepancy between experiment and theory as to the value of the Kondo temperature. We find that the ratio between the two Kondo temperatures in regime 1) and regime 2) is given by: $\mathcal{R}=\exp\left[\frac{π^{2}ρv_{F}}{2k_{F}^{2}Vol}\right]$ where $ρ$ is the density of states, $v_{F}$ is the fermi velocity, and $k_{F}$ is the Fermi wavevector and $Vol$ is the volume of a unit cell. We note that there is no dependence on the impurity concentration in this ratio so it is possible to define a single Kondo temperature for limit 2) for the dilute Kondo impurity system. In this work we present results within the Reed-Newns Kondo meanfield approximation and to leading order of the linked cluster expansion.
format Preprint
id arxiv_https___arxiv_org_abs_2410_05060
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Kondo Impurities at a Finite Concentration of Impurities
Goldstein, Garry
Strongly Correlated Electrons
Disordered Systems and Neural Networks
In this work we study the Kondo impurity problem - at a finite concentration of impurities. We identify two parameter regimes for the Kondo impurity problem. 1) The single impurity limit, where the concentration of Kondo impurities is so low that the background scattering mechanisms (non-magnetic impurities, Umklapp scattering, etc.) of the metal considered are the dominant conduction electron scattering mechanisms at zero temperature. 2) The dilute impurity system limit where the concentration of magnetic impurities is such that they form the dominant mechanism of conduction electron scattering at zero temperature of the metal in question (this is accompanied by a variety of easily detectable Kondo signatures (resistance minimum, specific heat measurements, magnetization as a function of external magnetic field, conduction electron dephasing rates as well as ARPES, RIXS and NMR spectroscopies)) while still being very dilute. Most theoretical efforts are currently in regime where a single isolated impurity is considered - regime 1) while most experimental efforts are in regime 2). We present analytical evidence that this explains the well known discrepancy between experiment and theory as to the value of the Kondo temperature. We find that the ratio between the two Kondo temperatures in regime 1) and regime 2) is given by: $\mathcal{R}=\exp\left[\frac{π^{2}ρv_{F}}{2k_{F}^{2}Vol}\right]$ where $ρ$ is the density of states, $v_{F}$ is the fermi velocity, and $k_{F}$ is the Fermi wavevector and $Vol$ is the volume of a unit cell. We note that there is no dependence on the impurity concentration in this ratio so it is possible to define a single Kondo temperature for limit 2) for the dilute Kondo impurity system. In this work we present results within the Reed-Newns Kondo meanfield approximation and to leading order of the linked cluster expansion.
title Kondo Impurities at a Finite Concentration of Impurities
topic Strongly Correlated Electrons
Disordered Systems and Neural Networks
url https://arxiv.org/abs/2410.05060