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Main Authors: Simon, C., Silevitch, D. M., Rosenbaum, T. F.
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2410.05556
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author Simon, C.
Silevitch, D. M.
Rosenbaum, T. F.
author_facet Simon, C.
Silevitch, D. M.
Rosenbaum, T. F.
contents We measure the non-linear magnetic susceptibility $χ^{(3)}$ of the disordered quantum Ising magnet, \lihofour, and demonstrate four-wave mixing due to coherent (anti-)Stokes Raman scattering at $\sim$ 100 Hz (p$e$V) energy scales. The temperature dependence of $χ^{(3)}$ approximately follows a $\frac{1}{T}$ form, with a high-$T$ cutoff that can be linked to dissipation in the coherent spin clusters. $χ^{(3)}$ also decreases monotonically with a transverse field, approaching a constant offset above a few kOe, suggesting the presence of both coherent, and spontaneous Raman scattering.
format Preprint
id arxiv_https___arxiv_org_abs_2410_05556
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Four-Wave Mixing at peV Energy Scales
Simon, C.
Silevitch, D. M.
Rosenbaum, T. F.
Strongly Correlated Electrons
We measure the non-linear magnetic susceptibility $χ^{(3)}$ of the disordered quantum Ising magnet, \lihofour, and demonstrate four-wave mixing due to coherent (anti-)Stokes Raman scattering at $\sim$ 100 Hz (p$e$V) energy scales. The temperature dependence of $χ^{(3)}$ approximately follows a $\frac{1}{T}$ form, with a high-$T$ cutoff that can be linked to dissipation in the coherent spin clusters. $χ^{(3)}$ also decreases monotonically with a transverse field, approaching a constant offset above a few kOe, suggesting the presence of both coherent, and spontaneous Raman scattering.
title Four-Wave Mixing at peV Energy Scales
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2410.05556